Open Access
Proceedings of the National Academy of Sciences of the United States of America, volume 106, issue 9, pages 3011-3016
Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics
1
Department of Chemistry, 80 Saint George Street, Institute for Optical Sciences, and Center for Quantum Information and Quantum Control, University of Toronto, Toronto, ON, Canada M5S 3H6
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Publication type: Journal Article
Publication date: 2009-02-13
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 11.1
ISSN: 00278424, 10916490
PubMed ID:
19218443
Multidisciplinary
Abstract
Charge carrier trapping is an important phenomenon in nanocrystal (NC) decay dynamics because it reduces photoluminescence (PL) quantum efficiencies and obscures efforts to understand the interaction of NC excitons with their surroundings. Particularly crucial to our understanding of excitation dynamics in, e.g., multiNC assemblies, would be a way of differentiating between processes involving trap states and those that do not. Direct optical measurement of NC trap state processes is not usually possible because they have negligible transition dipole moments; however, they are known to indirectly affect exciton photoluminescence. Here, we develop a framework, based on Marcus electron transfer theory, to determine NC trap state dynamics from time-resolved NC exciton PL measurements. Our results demonstrate the sensitivity of PL to interfacial dynamics, indicating that the technique can be used as an indirect but effective probe of trap distribution changes. We anticipate that this study represents a step toward understanding how excitons in nanocrystals interact with their surroundings: a quality that must be optimized for their efficient application in photovoltaics, photodetectors, or chemical sensors.
Top-30
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4 publications, 1.27%
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3 publications, 0.95%
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Chemical Physics Letters
3 publications, 0.95%
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3 publications, 0.95%
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3 publications, 0.95%
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3 publications, 0.95%
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3 publications, 0.95%
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2 publications, 0.63%
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2 publications, 0.63%
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2 publications, 0.63%
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2 publications, 0.63%
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2 publications, 0.63%
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Nanotechnology
2 publications, 0.63%
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Citations by publishers
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160
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American Chemical Society (ACS)
156 publications, 49.37%
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Elsevier
33 publications, 10.44%
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Wiley
28 publications, 8.86%
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Royal Society of Chemistry (RSC)
28 publications, 8.86%
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Springer Nature
14 publications, 4.43%
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American Institute of Physics (AIP)
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American Physical Society (APS)
10 publications, 3.16%
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IOP Publishing
7 publications, 2.22%
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Multidisciplinary Digital Publishing Institute (MDPI)
3 publications, 0.95%
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National Academy of Sciences of Ukraine (Co. LTD Ukrinformnauka) (Publications)
2 publications, 0.63%
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Annual Reviews
2 publications, 0.63%
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SPIE
2 publications, 0.63%
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CSIRO Publishing
1 publication, 0.32%
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Uspekhi Fizicheskikh Nauk Journal
1 publication, 0.32%
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Japan Society for Analytical Chemistry
1 publication, 0.32%
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Cambridge University Press
1 publication, 0.32%
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IEEE
1 publication, 0.32%
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Optical Society of America
1 publication, 0.32%
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American Association for the Advancement of Science (AAAS)
1 publication, 0.32%
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Proceedings of the National Academy of Sciences (PNAS)
1 publication, 0.32%
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Pleiades Publishing
1 publication, 0.32%
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Chinese Physical Society
1 publication, 0.32%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.32%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Jones M., Lo S. S., Scholes G. D. Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics // Proceedings of the National Academy of Sciences of the United States of America. 2009. Vol. 106. No. 9. pp. 3011-3016.
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Jones M., Lo S. S., Scholes G. D. Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics // Proceedings of the National Academy of Sciences of the United States of America. 2009. Vol. 106. No. 9. pp. 3011-3016.
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TY - JOUR
DO - 10.1073/pnas.0809316106
UR - https://doi.org/10.1073/pnas.0809316106
TI - Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics
T2 - Proceedings of the National Academy of Sciences of the United States of America
AU - Jones, Marcus
AU - Lo, Shun S
AU - Scholes, Gregory D.
PY - 2009
DA - 2009/02/13 00:00:00
PB - Proceedings of the National Academy of Sciences (PNAS)
SP - 3011-3016
IS - 9
VL - 106
PMID - 19218443
SN - 0027-8424
SN - 1091-6490
ER -
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@article{2009_Jones,
author = {Marcus Jones and Shun S Lo and Gregory D. Scholes},
title = {Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
year = {2009},
volume = {106},
publisher = {Proceedings of the National Academy of Sciences (PNAS)},
month = {feb},
url = {https://doi.org/10.1073/pnas.0809316106},
number = {9},
pages = {3011--3016},
doi = {10.1073/pnas.0809316106}
}
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Jones, Marcus, et al. “Quantitative modeling of the role of surface traps in CdSe/CdS/ZnS nanocrystal photoluminescence decay dynamics.” Proceedings of the National Academy of Sciences of the United States of America, vol. 106, no. 9, Feb. 2009, pp. 3011-3016. https://doi.org/10.1073/pnas.0809316106.