Nanotechnology, volume 17, issue 4, pages 956-962

Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals

Mark J. Fernée

Elizabeth Thomsen ¹

Peter Jensen ¹

H. Rubinsztein-Dunlop ¹

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Centre for Quantum Computer Technology, School of Physical Sciences, The University of Queensland, Queensland, 4072, Australia |

Publication type: Journal Article

Publication date: 2006-01-30

IOP Publishing

Journal: Nanotechnology

Quartile SCImago

Quartile WOS

Impact factor: 3.5

ISSN: 09574484, 13616528

DOI: 10.1088/0957-4484/17/4/020

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General Chemistry

General Materials Science

Electrical and Electronic Engineering

Mechanical Engineering

Bioengineering

Mechanics of Materials

Abstract

We report that high quality PbS nanocrystals, synthesized in the strong quantum confinement regime, have quantum yields as high as 70% at room temperature. We use a combination of modelling and photoluminescence up-conversion to show that we obtain a nearly monodisperse size distribution. Nevertheless, the emission displays a large nonresonant Stokes shift. The magnitude of the Stokes shift is found to be directly proportional to the degree of quantum confinement, from which we establish that the emission results from the recombination of one quantum confined charge carrier with one localized or surface-trapped charge carrier. Furthermore, the surface state energy is found to lie outside the bulk bandgap so that surface-related emission only commences for strongly quantum confined nanocrystals, thus highlighting a regime where improved surface passivation becomes necessary.

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Citations by journals

	1 2 3 4 5 6 7
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 7, 10% Journal of Physical Chemistry C 7 publications, 10%
ACS Nano	ACS Nano, 5, 7.14% ACS Nano 5 publications, 7.14%
Nanotechnology	Nanotechnology, 4, 5.71% Nanotechnology 4 publications, 5.71%
Applied Physics Letters	Applied Physics Letters, 3, 4.29% Applied Physics Letters 3 publications, 4.29%
Journal of Applied Physics	Journal of Applied Physics, 3, 4.29% Journal of Applied Physics 3 publications, 4.29%
Journal of Luminescence	Journal of Luminescence, 3, 4.29% Journal of Luminescence 3 publications, 4.29%
Nanoscale	Nanoscale, 3, 4.29% Nanoscale 3 publications, 4.29%
Physical Review B	Physical Review B, 2, 2.86% Physical Review B 2 publications, 2.86%
Nano Letters	Nano Letters, 2, 2.86% Nano Letters 2 publications, 2.86%
Micro and Nano Letters	Micro and Nano Letters, 1, 1.43% Micro and Nano Letters 1 publication, 1.43%
Optical and Quantum Electronics	Optical and Quantum Electronics, 1, 1.43% Optical and Quantum Electronics 1 publication, 1.43%
Nature Methods	Nature Methods, 1, 1.43% Nature Methods 1 publication, 1.43%
MRS Proceedings	MRS Proceedings, 1, 1.43% MRS Proceedings 1 publication, 1.43%
Analytical and Bioanalytical Chemistry	Analytical and Bioanalytical Chemistry, 1, 1.43% Analytical and Bioanalytical Chemistry 1 publication, 1.43%
Physica Scripta	Physica Scripta, 1, 1.43% Physica Scripta 1 publication, 1.43%
Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms	Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms, 1, 1.43% Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms 1 publication, 1.43%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 1.43% Journal of Alloys and Compounds 1 publication, 1.43%
Physica E: Low-Dimensional Systems and Nanostructures	Physica E: Low-Dimensional Systems and Nanostructures, 1, 1.43% Physica E: Low-Dimensional Systems and Nanostructures 1 publication, 1.43%
Materials Chemistry and Physics	Materials Chemistry and Physics, 1, 1.43% Materials Chemistry and Physics 1 publication, 1.43%
International Journal of Applied Glass Science	International Journal of Applied Glass Science, 1, 1.43% International Journal of Applied Glass Science 1 publication, 1.43%
Proteomics	Proteomics, 1, 1.43% Proteomics 1 publication, 1.43%
Advanced Energy Materials	Advanced Energy Materials, 1, 1.43% Advanced Energy Materials 1 publication, 1.43%
physica status solidi (c)	physica status solidi (c), 1, 1.43% physica status solidi (c) 1 publication, 1.43%
Journal of Physical Chemistry B	Journal of Physical Chemistry B, 1, 1.43% Journal of Physical Chemistry B 1 publication, 1.43%
Langmuir	Langmuir, 1, 1.43% Langmuir 1 publication, 1.43%
Chemistry of Materials	Chemistry of Materials, 1, 1.43% Chemistry of Materials 1 publication, 1.43%
Analytical Chemistry	Analytical Chemistry, 1, 1.43% Analytical Chemistry 1 publication, 1.43%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 1, 1.43% Journal of Physical Chemistry Letters 1 publication, 1.43%
ACS Energy Letters	ACS Energy Letters, 1, 1.43% ACS Energy Letters 1 publication, 1.43%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25
American Chemical Society (ACS)	American Chemical Society (ACS), 23, 32.86% American Chemical Society (ACS) 23 publications, 32.86%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 7, 10% American Institute of Physics (AIP) 7 publications, 10%
Elsevier	Elsevier, 7, 10% Elsevier 7 publications, 10%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 6, 8.57% Royal Society of Chemistry (RSC) 6 publications, 8.57%
IOP Publishing	IOP Publishing, 5, 7.14% IOP Publishing 5 publications, 7.14%
Springer Nature	Springer Nature, 4, 5.71% Springer Nature 4 publications, 5.71%
Wiley	Wiley, 4, 5.71% Wiley 4 publications, 5.71%
American Physical Society (APS)	American Physical Society (APS), 2, 2.86% American Physical Society (APS) 2 publications, 2.86%
Taylor & Francis	Taylor & Francis, 2, 2.86% Taylor & Francis 2 publications, 2.86%
Institution of Engineering and Technology (IET)	Institution of Engineering and Technology (IET), 1, 1.43% Institution of Engineering and Technology (IET) 1 publication, 1.43%
Materials Research Society	Materials Research Society, 1, 1.43% Materials Research Society 1 publication, 1.43%
Pleiades Publishing	Pleiades Publishing, 1, 1.43% Pleiades Publishing 1 publication, 1.43%
Optical Society of America	Optical Society of America, 1, 1.43% Optical Society of America 1 publication, 1.43%
Trans Tech Publications	Trans Tech Publications, 1, 1.43% Trans Tech Publications 1 publication, 1.43%
SPIE	SPIE, 1, 1.43% SPIE 1 publication, 1.43%
IEEE	IEEE, 1, 1.43% IEEE 1 publication, 1.43%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.43% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.43%
	5 10 15 20 25

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
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Fernée M. J. et al. Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals // Nanotechnology. 2006. Vol. 17. No. 4. pp. 956-962.

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Fernée M. J., Thomsen E., Jensen P., Rubinsztein-Dunlop H. Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals // Nanotechnology. 2006. Vol. 17. No. 4. pp. 956-962.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1088/0957-4484/17/4/020

UR - https://doi.org/10.1088/0957-4484/17/4/020

TI - Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals

T2 - Nanotechnology

AU - Fernée, Mark J.

AU - Thomsen, Elizabeth

AU - Jensen, Peter

AU - Rubinsztein-Dunlop, H.

PY - 2006

DA - 2006/01/30 00:00:00

PB - IOP Publishing

SP - 956-962

IS - 4

VL - 17

SN - 0957-4484

SN - 1361-6528

ER -

BibTex |

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BibTex Copy

@article{2006_Fernée,

author = {Mark J. Fernée and Elizabeth Thomsen and Peter Jensen and H. Rubinsztein-Dunlop},

title = {Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals},

journal = {Nanotechnology},

year = {2006},

volume = {17},

publisher = {IOP Publishing},

month = {jan},

url = {https://doi.org/10.1088/0957-4484/17/4/020},

number = {4},

pages = {956--962},

doi = {10.1088/0957-4484/17/4/020}

}

MLA

Cite this

MLA Copy

Fernée, Mark J., et al. “Highly efficient luminescence from a hybrid state found in strongly quantum confined PbS nanocrystals.” Nanotechnology, vol. 17, no. 4, Jan. 2006, pp. 956-962. https://doi.org/10.1088/0957-4484/17/4/020.

Found error?

Publisher

IOP Publishing

Journal

Nanotechnology

Quartile SCImago

Quartile WOS

Impact factor

3.5

ISSN

09574484 (Print)
13616528 (Electronic)