Open Access

Physical Review Letters, volume 126, issue 17, publication number 175501

High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph

Maxim Bykov ^{1, 2}

Timofey Fedotenko ³

Stella Chariton ⁴

Dominique Laniel ³

K. Glazyrin ⁵

M. Hanfland ⁶

Jesse J. Smith ⁷

Jesse S. Smith ⁷

V. Prakapenka ⁴

Mohammad F. Mahmood ¹

Alexander Goncharov ²

Alexander F. Goncharov ²

A.V. Ponomareva ⁸

Ferenc Tasnádi ⁹

F. Tasnádi ⁹

Alexei I Abrikosov ¹⁰

A.A. Abrikosov ¹⁰

Talha Bin Masood ¹⁰

Ingrid Hotz ¹⁰

Alexander N Rudenko ^{11, 12, 13}

Alexander N. Rudenko ^{11, 12, 13}

Mikhail I Katsnelson ^{11, 13}

M. I. KATSNELSON ^{11, 13}

N.A. Dubrovinskaia ^{3, 9}

Leonid Dubrovinsky ¹⁴

L. Dubrovinsky ¹⁴

Igor A Abrikosov ⁹

I. A. Abrikosov ⁹

Hide authors affiliations Show authors affiliations: 14 affiliations

College of Arts and Science, Howard University, Washington, D.C. 20059, USA |

The Earth and Planets Laboratory, Carnegie Institution for Science, Washington, D.C. 20015, USA |

Material Physics and Technology at Extreme Conditions, Laboratory of Crystallography, University of Bayreuth, 95440 Bayreuth, Germany |

⁴

Center for Advanced Radiation Sources, University of Chicago, Chicago, Illinois 60637, USA |

⁵

Photon Sciences, Deutsches Electronen Synchrotron (DESY), D-22607 Hamburg, Germany |

⁶

European Synchrotron Radiation Facility, 38043 Grenoble Cedex 9, France |

⁷

HPCAT, X-Ray Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA |

⁸

Materials Modeling and Development Laboratory, National University of Science and Technology “MISiS,” 119049 Moscow, Russia |

⁹

Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-58183 Linköping, Sweden |

¹⁰

Department of Science and Technology (ITN), Linköping University, SE-60174 Norrköping, Sweden |

¹¹

Radboud University, Institute for Molecules and Materials, 6525AJ Nijmegen, The Netherlands |

¹²

Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education and School of Physics and Technology, Wuhan University, Wuhan 430072, China |

¹³

Department of Theoretical Physics and Applied Mathematics, Ural Federal University, 620002 Ekaterinburg, Russia |

¹⁴

Bayerisches Geoinstitut, University of Bayreuth, 95440 Bayreuth, Germany |

Publication type: Journal Article

Publication date: 2021-04-26

American Physical Society (APS)

Journal: Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 00319007, 10797114

DOI: 10.1103/PhysRevLett.126.175501

Copy DOI

General Physics and Astronomy

Abstract

High pressure chemistry is known to inspire the creation of unexpected new classes of compounds with exceptional properties. Here we report the synthesis at ~90 GPa of novel beryllium polynitrides, monoclinic and triclinic BeN4. The triclinic phase, upon decompression to ambient conditions, transforms into a compound with atomic-thick BeN4 layers interconnected via weak van der Waals bonds consisting of polyacetylene-like nitrogen chains with conjugated {\pi}-systems and Be atoms in square-planar coordination. Theoretical calculations for a single BeN4 layer show that its electronic lattice is described by a slightly distorted honeycomb structure reminiscent of the graphene lattice and the presence of Dirac points in the electronic band structure at the Fermi level. The BeN4 layer, i.e. beryllonitrene, represents a qualitatively new class of 2D materials that can be built of a metal atom and polymeric nitrogen chains and host anisotropic Dirac fermions.

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Citations by journals

	1 2 3 4 5
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 5, 5.21% Physical Chemistry Chemical Physics 5 publications, 5.21%
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Journal of the American Chemical Society	Journal of the American Chemical Society, 3, 3.13% Journal of the American Chemical Society 3 publications, 3.13%
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Physica E: Low-Dimensional Systems and Nanostructures	Physica E: Low-Dimensional Systems and Nanostructures, 2, 2.08% Physica E: Low-Dimensional Systems and Nanostructures 2 publications, 2.08%
2D Materials	2D Materials, 2, 2.08% 2D Materials 2 publications, 2.08%
Angewandte Chemie	Angewandte Chemie, 2, 2.08% Angewandte Chemie 2 publications, 2.08%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 2, 2.08% Angewandte Chemie - International Edition 2 publications, 2.08%
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ACS Omega	ACS Omega, 2, 2.08% ACS Omega 2 publications, 2.08%
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Nature Chemistry	Nature Chemistry, 1, 1.04% Nature Chemistry 1 publication, 1.04%
Applied Physics Letters	Applied Physics Letters, 1, 1.04% Applied Physics Letters 1 publication, 1.04%
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Communications Chemistry	Communications Chemistry, 1, 1.04% Communications Chemistry 1 publication, 1.04%
FlatChem	FlatChem, 1, 1.04% FlatChem 1 publication, 1.04%
Physics Letters, Section A: General, Atomic and Solid State Physics	Physics Letters, Section A: General, Atomic and Solid State Physics, 1, 1.04% Physics Letters, Section A: General, Atomic and Solid State Physics 1 publication, 1.04%
Results in Physics	Results in Physics, 1, 1.04% Results in Physics 1 publication, 1.04%
ChemPhysMater	ChemPhysMater, 1, 1.04% ChemPhysMater 1 publication, 1.04%
Solid State Communications	Solid State Communications, 1, 1.04% Solid State Communications 1 publication, 1.04%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 1, 1.04% Journal of Alloys and Compounds 1 publication, 1.04%
Nano-Structures and Nano-Objects	Nano-Structures and Nano-Objects, 1, 1.04% Nano-Structures and Nano-Objects 1 publication, 1.04%
Applied Physics Express	Applied Physics Express, 1, 1.04% Applied Physics Express 1 publication, 1.04%
	1 2 3 4 5

Citations by publishers

	5 10 15 20 25 30
Elsevier	Elsevier, 27, 28.13% Elsevier 27 publications, 28.13%
American Chemical Society (ACS)	American Chemical Society (ACS), 15, 15.63% American Chemical Society (ACS) 15 publications, 15.63%
IOP Publishing	IOP Publishing, 13, 13.54% IOP Publishing 13 publications, 13.54%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 10, 10.42% Royal Society of Chemistry (RSC) 10 publications, 10.42%
Wiley	Wiley, 7, 7.29% Wiley 7 publications, 7.29%
American Physical Society (APS)	American Physical Society (APS), 7, 7.29% American Physical Society (APS) 7 publications, 7.29%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 6, 6.25% American Institute of Physics (AIP) 6 publications, 6.25%
Springer Nature	Springer Nature, 5, 5.21% Springer Nature 5 publications, 5.21%
International Union of Crystallography (IUCr)	International Union of Crystallography (IUCr), 1, 1.04% International Union of Crystallography (IUCr) 1 publication, 1.04%
Japan Society of Applied Physics	Japan Society of Applied Physics, 1, 1.04% Japan Society of Applied Physics 1 publication, 1.04%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.04% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.04%
	5 10 15 20 25 30

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Bykov M. et al. High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph // Physical Review Letters. 2021. Vol. 126. No. 17. 175501

GOST all authors (up to 50) Copy

Bykov M., Fedotenko T., Chariton S., Laniel D., Glazyrin K., Hanfland M., Smith J. J., Smith J. S., Prakapenka V., Mahmood M. F., Goncharov A., Goncharov A. F., Ponomareva A., Tasnádi F., Tasnádi F., Abrikosov A., Abrikosov A. I., Masood T. B., Bin Masood T., Hotz I., Rudenko A. N., Rudenko A. N., KATSNELSON M. I., Katsnelson M. I., Dubrovinskaia N., Dubrovinsky L., Dubrovinsky L., Abrikosov I. A., Abrikosov I. A. High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph // Physical Review Letters. 2021. Vol. 126. No. 17. 175501

RIS |

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RIS Copy

TY - JOUR

DO - 10.1103/PhysRevLett.126.175501

UR - https://doi.org/10.1103/PhysRevLett.126.175501

TI - High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph

T2 - Physical Review Letters

AU - Bykov, Maxim

AU - Fedotenko, Timofey

AU - Chariton, Stella

AU - Laniel, Dominique

AU - Glazyrin, K.

AU - Hanfland, M.

AU - Prakapenka, V.

AU - Mahmood, Mohammad F.

AU - Ponomareva, A.V.

AU - Tasnádi, Ferenc

AU - Abrikosov, Alexei I

AU - Bin Masood, Talha

AU - Hotz, Ingrid

AU - Rudenko, Alexander N

AU - Katsnelson, Mikhail I

AU - Dubrovinskaia, N.A.

AU - Dubrovinsky, Leonid

AU - Abrikosov, Igor A

AU - Smith, Jesse S.

AU - Goncharov, Alexander F.

AU - Smith, Jesse J.

AU - Goncharov, Alexander

AU - Tasnádi, F.

AU - Abrikosov, A.A.

AU - Masood, Talha Bin

AU - Rudenko, Alexander N.

AU - KATSNELSON, M. I.

AU - Dubrovinsky, L.

AU - Abrikosov, I. A.

PY - 2021

DA - 2021/04/26 00:00:00

PB - American Physical Society (APS)

IS - 17

VL - 126

SN - 0031-9007

SN - 1079-7114

ER -

BibTex

Cite this

BibTex Copy

@article{2021_Bykov,

author = {Maxim Bykov and Timofey Fedotenko and Stella Chariton and Dominique Laniel and K. Glazyrin and M. Hanfland and V. Prakapenka and Mohammad F. Mahmood and A.V. Ponomareva and Ferenc Tasnádi and Alexei I Abrikosov and Talha Bin Masood and Ingrid Hotz and Alexander N Rudenko and Mikhail I Katsnelson and N.A. Dubrovinskaia and Leonid Dubrovinsky and Igor A Abrikosov and Jesse S. Smith and Alexander F. Goncharov and Jesse J. Smith and Alexander Goncharov and F. Tasnádi and A.A. Abrikosov and Talha Bin Masood and Alexander N. Rudenko and M. I. KATSNELSON and L. Dubrovinsky and I. A. Abrikosov},

title = {High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph},

journal = {Physical Review Letters},

year = {2021},

volume = {126},

publisher = {American Physical Society (APS)},

month = {apr},

url = {https://doi.org/10.1103/PhysRevLett.126.175501},

number = {17},

doi = {10.1103/PhysRevLett.126.175501}

}

Found error?

Publisher

American Physical Society (APS)

Journal

Physical Review Letters

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

00319007 (Print)
10797114 (Electronic)

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