Open Access
Hydrogen Storage in Microporous Metal-Organic Frameworks
Тип публикации: Journal Article
Дата публикации: 2003-05-16
scimago Q1
wos Q1
БС1
SJR: 10.416
CiteScore: 48.4
Impact factor: 45.8
ISSN: 00368075, 10959203
PubMed ID:
12750515
Multidisciplinary
Краткое описание
Metal-organic framework-5 (MOF-5) of composition Zn 4 O(BDC) 3 (BDC = 1,4-benzenedicarboxylate) with a cubic three-dimensional extended porous structure adsorbed hydrogen up to 4.5 weight percent (17.2 hydrogen molecules per formula unit) at 78 kelvin and 1.0 weight percent at room temperature and pressure of 20 bar. Inelastic neutron scattering spectroscopy of the rotational transitions of the adsorbed hydrogen molecules indicates the presence of two well-defined binding sites (termed I and II), which we associate with hydrogen binding to zinc and the BDC linker, respectively. Preliminary studies on topologically similar isoreticular metal-organic framework-6 and -8 (IRMOF-6 and -8) having cyclobutylbenzene and naphthalene linkers, respectively, gave approximately double and quadruple (2.0 weight percent) the uptake found for MOF-5 at room temperature and 10 bar.
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ГОСТ
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Rosi N. L. et al. Hydrogen Storage in Microporous Metal-Organic Frameworks // Science. 2003. Vol. 300. No. 5622. pp. 1127-1129.
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Скопировать
Rosi N. L., Eckert J., Eddaoudi M., Vodak D. T., Kim J., O'Keeffe M., Yaghi O. M. Hydrogen Storage in Microporous Metal-Organic Frameworks // Science. 2003. Vol. 300. No. 5622. pp. 1127-1129.
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TY - JOUR
DO - 10.1126/science.1083440
UR - https://doi.org/10.1126/science.1083440
TI - Hydrogen Storage in Microporous Metal-Organic Frameworks
T2 - Science
AU - Rosi, Nathaniel L
AU - Eckert, Juergen
AU - Eddaoudi, Mohamed
AU - Vodak, David T
AU - Kim, Jaheon
AU - O'Keeffe, Michael
AU - Yaghi, Omar M.
PY - 2003
DA - 2003/05/16
PB - American Association for the Advancement of Science (AAAS)
SP - 1127-1129
IS - 5622
VL - 300
PMID - 12750515
SN - 0036-8075
SN - 1095-9203
ER -
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BibTex (до 50 авторов)
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@article{2003_Rosi,
author = {Nathaniel L Rosi and Juergen Eckert and Mohamed Eddaoudi and David T Vodak and Jaheon Kim and Michael O'Keeffe and Omar M. Yaghi},
title = {Hydrogen Storage in Microporous Metal-Organic Frameworks},
journal = {Science},
year = {2003},
volume = {300},
publisher = {American Association for the Advancement of Science (AAAS)},
month = {may},
url = {https://doi.org/10.1126/science.1083440},
number = {5622},
pages = {1127--1129},
doi = {10.1126/science.1083440}
}
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MLA
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Rosi, Nathaniel L., et al. “Hydrogen Storage in Microporous Metal-Organic Frameworks.” Science, vol. 300, no. 5622, May. 2003, pp. 1127-1129. https://doi.org/10.1126/science.1083440.