Open Access
Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation
Тип публикации: Journal Article
Дата публикации: 2003-08-08
scimago Q1
wos Q1
БС1
SJR: 10.416
CiteScore: 48.4
Impact factor: 45.8
ISSN: 00368075, 10959203
PubMed ID:
12907796
Multidisciplinary
Краткое описание
Acetic acid is an important petrochemical that is currently produced from methane (or coal) in a three-step process based on carbonylation of methanol. We report a direct, selective, oxidative condensation of two methane molecules to acetic acid at 180°C in liquid sulfuric acid. Carbon-13 isotopic labeling studies show that both carbons of acetic acid originate from methane. The reaction is catalyzed by palladium, and the results are consistent with the reaction occurring by tandem catalysis, involving methane C-H activation to generate Pd-CH 3 species, followed by efficient oxidative carbonylation with methanol, generated in situ from methane, to produce acetic acid.
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370
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MLA
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ГОСТ
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Periana R. A. et al. Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation // Science. 2003. Vol. 301. No. 5634. pp. 814-818.
ГОСТ со всеми авторами (до 50)
Скопировать
Periana R. A., Mironov O., Taube D., Bhalla G., Jones C. Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation // Science. 2003. Vol. 301. No. 5634. pp. 814-818.
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RIS
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TY - JOUR
DO - 10.1126/science.1086466
UR - https://doi.org/10.1126/science.1086466
TI - Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation
T2 - Science
AU - Periana, Roy A
AU - Mironov, Oleg
AU - Taube, Doug
AU - Bhalla, Gaurav
AU - Jones, CJ
PY - 2003
DA - 2003/08/08
PB - American Association for the Advancement of Science (AAAS)
SP - 814-818
IS - 5634
VL - 301
PMID - 12907796
SN - 0036-8075
SN - 1095-9203
ER -
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BibTex (до 50 авторов)
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@article{2003_Periana,
author = {Roy A Periana and Oleg Mironov and Doug Taube and Gaurav Bhalla and CJ Jones},
title = {Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation},
journal = {Science},
year = {2003},
volume = {301},
publisher = {American Association for the Advancement of Science (AAAS)},
month = {aug},
url = {https://doi.org/10.1126/science.1086466},
number = {5634},
pages = {814--818},
doi = {10.1126/science.1086466}
}
Цитировать
MLA
Скопировать
Periana, Roy A., et al. “Catalytic, Oxidative Condensation of CH 4 to CH 3 COOH in One Step via CH Activation.” Science, vol. 301, no. 5634, Aug. 2003, pp. 814-818. https://doi.org/10.1126/science.1086466.