Open Access

Science, volume 362, issue 6410, pages 69-72

Quantifying hot carrier and thermal contributions in plasmonic photocatalysis

Zhou Linan ¹

Swearer Dayne ¹

Zhang Chao ²

Robatjazi Hossein ²

Zhao Hangqi ²

Henderson Luke ¹

Dong Liangliang ¹

Christopher Phillip ³

Carter Emily A. ⁴

Nordlander Peter ^{2, 5}

Halas Naomi ^{1, 2, 5}

Hide authors affiliations Show authors affiliations: 5 affiliations

Department of Chemistry, Rice University, Houston, TX 77005, USA. |

Department of Electrical and Computer Engineering, Rice University, Houston, TX 77005, USA. |

Department of Chemical Engineering, University of California, Santa Barbara, Santa Barbara, CA, 93106-5080, USA. |

⁴

School of Engineering and Applied Science, Princeton University, Princeton, NJ 08544-5263, USA. |

⁵

Department of Physics and Astronomy, Rice University, Houston, TX 77005, USA. |

Publication type: Journal Article

Publication date: 2018-10-05

American Association for the Advancement of Science (AAAS)

Journal: Science

Quartile SCImago

Quartile WOS

Impact factor: 56.9

ISSN: 00368075, 10959203

DOI: 10.1126/science.aat6967

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Multidisciplinary

Abstract

Hot carriers reducing thermal barriers Plasmonic catalysts can generate hot charge carriers that can activate reactants and, in turn, reduce the overall barrier to a reaction. Zhou et al. studied the decomposition of ammonia to hydrogen on a copper alloy nanostructure that absorbed light and generated electrons that activated nitrogen atoms on ruthenium surface atoms (see the Perspective by Cortés). By measuring reaction rates at different wavelengths, light intensities, and catalyst surface temperatures, the light-induced reduction of the apparent activation barrier was quantified. Science, this issue p. 69; see also p. 28 A Ru-Cu alloy plasmonic photocatalyst substantially reduced the thermal activation barrier for ammonia decomposition. Photocatalysis based on optically active, “plasmonic” metal nanoparticles has emerged as a promising approach to facilitate light-driven chemical conversions under far milder conditions than thermal catalysis. However, an understanding of the relation between thermal and electronic excitations has been lacking. We report the substantial light-induced reduction of the thermal activation barrier for ammonia decomposition on a plasmonic photocatalyst. We introduce the concept of a light-dependent activation barrier to account for the effect of light illumination on electronic and thermal excitations in a single unified picture. This framework provides insight into the specific role of hot carriers in plasmon-mediated photochemistry, which is critically important for designing energy-efficient plasmonic photocatalysts.

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Citations by journals

	5 10 15 20 25 30 35 40
Nano Letters	Nano Letters, 37, 5.03% Nano Letters 37 publications, 5.03%
ACS Nano	ACS Nano, 36, 4.89% ACS Nano 36 publications, 4.89%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 32, 4.35% Journal of Physical Chemistry C 32 publications, 4.35%
Journal of the American Chemical Society	Journal of the American Chemical Society, 23, 3.13% Journal of the American Chemical Society 23 publications, 3.13%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 21, 2.85% Applied Catalysis B: Environmental 21 publications, 2.85%
ACS applied materials & interfaces	ACS applied materials & interfaces, 20, 2.72% ACS applied materials & interfaces 20 publications, 2.72%
ACS Catalysis	ACS Catalysis, 18, 2.45% ACS Catalysis 18 publications, 2.45%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 17, 2.31% Angewandte Chemie - International Edition 17 publications, 2.31%
Angewandte Chemie	Angewandte Chemie, 17, 2.31% Angewandte Chemie 17 publications, 2.31%
Nanoscale	Nanoscale, 15, 2.04% Nanoscale 15 publications, 2.04%
ACS Energy Letters	ACS Energy Letters, 15, 2.04% ACS Energy Letters 15 publications, 2.04%
Chemical Engineering Journal	Chemical Engineering Journal, 14, 1.9% Chemical Engineering Journal 14 publications, 1.9%
Chemical Science	Chemical Science, 13, 1.77% Chemical Science 13 publications, 1.77%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 13, 1.77% Journal of Physical Chemistry Letters 13 publications, 1.77%
ACS Photonics	ACS Photonics, 13, 1.77% ACS Photonics 13 publications, 1.77%
Nature Communications	Nature Communications, 12, 1.63% Nature Communications 12 publications, 1.63%
Accounts of Chemical Research	Accounts of Chemical Research, 10, 1.36% Accounts of Chemical Research 10 publications, 1.36%
Small	Small, 10, 1.36% Small 10 publications, 1.36%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 10, 1.36% Physical Chemistry Chemical Physics 10 publications, 1.36%
Advanced Materials	Advanced Materials, 9, 1.22% Advanced Materials 9 publications, 1.22%
Journal of Chemical Physics	Journal of Chemical Physics, 9, 1.22% Journal of Chemical Physics 9 publications, 1.22%
Advanced Functional Materials	Advanced Functional Materials, 9, 1.22% Advanced Functional Materials 9 publications, 1.22%
Chemical Communications	Chemical Communications, 9, 1.22% Chemical Communications 9 publications, 1.22%
Proceedings of the National Academy of Sciences of the United States of America	Proceedings of the National Academy of Sciences of the United States of America, 9, 1.22% Proceedings of the National Academy of Sciences of the United States of America 9 publications, 1.22%
ACS Applied Nano Materials	ACS Applied Nano Materials, 8, 1.09% ACS Applied Nano Materials 8 publications, 1.09%
Nano Energy	Nano Energy, 8, 1.09% Nano Energy 8 publications, 1.09%
Journal of Applied Physics	Journal of Applied Physics, 7, 0.95% Journal of Applied Physics 7 publications, 0.95%
Nanophotonics	Nanophotonics, 7, 0.95% Nanophotonics 7 publications, 0.95%
Science	Science, 6, 0.82% Science 6 publications, 0.82%
	5 10 15 20 25 30 35 40

Citations by publishers

	50 100 150 200 250 300
American Chemical Society (ACS)	American Chemical Society (ACS), 258, 35.05% American Chemical Society (ACS) 258 publications, 35.05%
Elsevier	Elsevier, 113, 15.35% Elsevier 113 publications, 15.35%
Wiley	Wiley, 100, 13.59% Wiley 100 publications, 13.59%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 84, 11.41% Royal Society of Chemistry (RSC) 84 publications, 11.41%
Springer Nature	Springer Nature, 56, 7.61% Springer Nature 56 publications, 7.61%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 27, 3.67% American Institute of Physics (AIP) 27 publications, 3.67%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 14, 1.9% Multidisciplinary Digital Publishing Institute (MDPI) 14 publications, 1.9%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 11, 1.49% American Association for the Advancement of Science (AAAS) 11 publications, 1.49%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 9, 1.22% Proceedings of the National Academy of Sciences (PNAS) 9 publications, 1.22%
Walter de Gruyter	Walter de Gruyter, 8, 1.09% Walter de Gruyter 8 publications, 1.09%
Optical Society of America	Optical Society of America, 7, 0.95% Optical Society of America 7 publications, 0.95%
Chinese Physical Society	Chinese Physical Society, 5, 0.68% Chinese Physical Society 5 publications, 0.68%
American Physical Society (APS)	American Physical Society (APS), 4, 0.54% American Physical Society (APS) 4 publications, 0.54%
IOP Publishing	IOP Publishing, 4, 0.54% IOP Publishing 4 publications, 0.54%
Oxford University Press	Oxford University Press, 3, 0.41% Oxford University Press 3 publications, 0.41%
Annual Reviews	Annual Reviews, 3, 0.41% Annual Reviews 3 publications, 0.41%
Cambridge University Press	Cambridge University Press, 2, 0.27% Cambridge University Press 2 publications, 0.27%
Pleiades Publishing	Pleiades Publishing, 2, 0.27% Pleiades Publishing 2 publications, 0.27%
Taylor & Francis	Taylor & Francis, 2, 0.27% Taylor & Francis 2 publications, 0.27%
SPIE	SPIE, 1, 0.14% SPIE 1 publication, 0.14%
World Scientific	World Scientific, 1, 0.14% World Scientific 1 publication, 0.14%
The Electrochemical Society	The Electrochemical Society, 1, 0.14% The Electrochemical Society 1 publication, 0.14%
SAGE	SAGE, 1, 0.14% SAGE 1 publication, 0.14%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.14% Frontiers Media S.A. 1 publication, 0.14%
Japan Society of Applied Physics	Japan Society of Applied Physics, 1, 0.14% Japan Society of Applied Physics 1 publication, 0.14%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.14% Taiwan Institute of Chemical Engineers 1 publication, 0.14%
Social Science Electronic Publishing	Social Science Electronic Publishing, 1, 0.14% Social Science Electronic Publishing 1 publication, 0.14%
Science in China Press	Science in China Press, 1, 0.14% Science in China Press 1 publication, 0.14%
Cairo University	Cairo University, 1, 0.14% Cairo University 1 publication, 0.14%
	50 100 150 200 250 300

We do not take into account publications that without a DOI.
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Zhou L. et al. Quantifying hot carrier and thermal contributions in plasmonic photocatalysis // Science. 2018. Vol. 362. No. 6410. pp. 69-72.

GOST all authors (up to 50) Copy

Zhou L., Swearer D., Zhang C., Robatjazi H., Zhao H., Henderson L., Dong L., Christopher P., Carter E. A., Nordlander P., Halas N. Quantifying hot carrier and thermal contributions in plasmonic photocatalysis // Science. 2018. Vol. 362. No. 6410. pp. 69-72.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1126/science.aat6967

UR - https://doi.org/10.1126%2Fscience.aat6967

TI - Quantifying hot carrier and thermal contributions in plasmonic photocatalysis

T2 - Science

AU - Zhou, Linan

AU - Swearer, Dayne

AU - Robatjazi, Hossein

AU - Zhao, Hangqi

AU - Henderson, Luke

AU - Dong, Liangliang

AU - Carter, Emily A.

AU - Nordlander, Peter

AU - Halas, Naomi

AU - Zhang, Chao

AU - Christopher, Phillip

PY - 2018

DA - 2018/10/05 00:00:00

PB - American Association for the Advancement of Science (AAAS)

SP - 69-72

IS - 6410

VL - 362

SN - 0036-8075

SN - 1095-9203

ER -

BibTex |

Cite this

BibTex Copy

@article{2018_Zhou,

author = {Linan Zhou and Dayne Swearer and Hossein Robatjazi and Hangqi Zhao and Luke Henderson and Liangliang Dong and Emily A. Carter and Peter Nordlander and Naomi Halas and Chao Zhang and Phillip Christopher},

title = {Quantifying hot carrier and thermal contributions in plasmonic photocatalysis},

journal = {Science},

year = {2018},

volume = {362},

publisher = {American Association for the Advancement of Science (AAAS)},

month = {oct},

url = {https://doi.org/10.1126%2Fscience.aat6967},

number = {6410},

pages = {69--72},

doi = {10.1126/science.aat6967}

}

MLA

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MLA Copy

Zhou, Linan, et al. “Quantifying hot carrier and thermal contributions in plasmonic photocatalysis.” Science, vol. 362, no. 6410, Oct. 2018, pp. 69-72. https://doi.org/10.1126%2Fscience.aat6967.

Found error?

Publisher

American Association for the Advancement of Science (AAAS)

Journal

Science

Quartile SCImago

Quartile WOS

Impact factor

56.9

ISSN

00368075 (Print)
10959203 (Electronic)

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