Journal of the Electrochemical Society, volume 161, issue 12, pages A1812-A1817
Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor
1
Department of Mechanical Engineering, University of Colorado at Boulder, Boulder, Colorado 80309-0427, USA
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Publication type: Journal Article
Publication date: 2014-08-22
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.9
ISSN: 00134651, 19457111
Materials Chemistry
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Electrochemistry
Condensed Matter Physics
Renewable Energy, Sustainability and the Environment
Abstract
Replacing the liquid electrolyte in a lithium battery with a solid electrolyte can resolve many inherent safety issues as well as enable the use of next generation electrode materials. Recent research in solid electrolytes, however, has mainly focused on improving ionic conductivity while neglecting compatibility with energy dense anodes such as lithium metal. Herein, we report a new crystalline solid electrolyte devised to be inexpensive, highly conductive, and compatible with lithium metal. This study presents and characterizes an analog to Li10GeP2S12 using the isovalent ion of silicon to displace germanium as a cost effective constituent. The crystal Li10SiP2S12 displays a conductivity of 2.3 × 10−3 S cm−1, the highest reported conductivity for an unsintered silicon-based solid electrolyte. Impedance spectroscopy is used to probe interactions between the new superionic conductor and lithium metal revealing a more favorable decomposition than previous metal containing electrolytes. Due to the enhanced compatibility of Li10SiP2S12 with lithium metal, we present one of the longest cycling bulk solid-state lithium metal batteries to date. Discerning the nature of chemical decomposition at the electrolyte-lithium interface is essential to the design and synthesis of future solid electrolytes.
Top-30
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Citations by publishers
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5
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25
30
35
40
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Elsevier
40 publications, 27.59%
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American Chemical Society (ACS)
29 publications, 20%
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Wiley
24 publications, 16.55%
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Springer Nature
14 publications, 9.66%
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3 publications, 2.07%
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2 publications, 1.38%
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Walter de Gruyter
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OAE Publishing Inc.
2 publications, 1.38%
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Taylor & Francis
1 publication, 0.69%
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ASME
1 publication, 0.69%
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American Vacuum Society
1 publication, 0.69%
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International Union of Crystallography (IUCr)
1 publication, 0.69%
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The Electrochemical Society
1 publication, 0.69%
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Japan Institute of Metals and Materials
1 publication, 0.69%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 0.69%
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University of Science and Technology Beijing
1 publication, 0.69%
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Cambridge University Press
1 publication, 0.69%
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Japan Society of Applied Physics
1 publication, 0.69%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.69%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Whiteley J. M. et al. Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor // Journal of the Electrochemical Society. 2014. Vol. 161. No. 12. p. A1812-A1817.
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Whiteley J. M., Woo J. H., Hu E., Nam K., Lee S. Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor // Journal of the Electrochemical Society. 2014. Vol. 161. No. 12. p. A1812-A1817.
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TY - JOUR
DO - 10.1149/2.0501412jes
UR - https://doi.org/10.1149/2.0501412jes
TI - Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor
T2 - Journal of the Electrochemical Society
AU - Whiteley, Justin M.
AU - Woo, Jae H.
AU - Hu, Enyuan
AU - Nam, Kyung-Wan
AU - Lee, Se-Hee
PY - 2014
DA - 2014/08/22 00:00:00
PB - The Electrochemical Society
SP - A1812-A1817
IS - 12
VL - 161
SN - 0013-4651
SN - 1945-7111
ER -
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@article{2014_Whiteley,
author = {Justin M. Whiteley and Jae H. Woo and Enyuan Hu and Kyung-Wan Nam and Se-Hee Lee},
title = {Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor},
journal = {Journal of the Electrochemical Society},
year = {2014},
volume = {161},
publisher = {The Electrochemical Society},
month = {aug},
url = {https://doi.org/10.1149/2.0501412jes},
number = {12},
pages = {A1812--A1817},
doi = {10.1149/2.0501412jes}
}
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MLA
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Whiteley, Justin M., et al. “Empowering the Lithium Metal Battery through a Silicon-Based Superionic Conductor.” Journal of the Electrochemical Society, vol. 161, no. 12, Aug. 2014, pp. A1812-A1817. https://doi.org/10.1149/2.0501412jes.