Enhanced terahertz emission from imprinted halide perovskite nanostructures
Lead halide perovskites were known to be a prospective family of materials for terahertz (THz) generation. On the other hand, perovskite nanostructures, nanoantennas, and metasurfaces allow tailoring perovskites optical characteristics, resulting in more efficient interaction with incident or emitted light. Moreover, the perovskites are robust materials against formation of defects caused by mechanical deformations and can be efficiently nanostructured by various high throughput methods. In this work, we have enhanced THz emission from MAPbI3 perovskite upon femtosecond laser irradiation using nanoimprint lithography. The formed nanostructures not only improve absorption of the incident laser pulses, but also lead to a non-symmetric near-field distribution. As a result, we have enhanced the efficiency of THz emission from the nanostructured perovskite by 3.5 times as compared with a smooth perovskite film. Our results paved the way for a new application of large-scale perovskite nanostructuring, making halide perovskites competitive with more expensive conventional semiconductors for THz generation.
Citations by journals
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Nanoscale
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JETP Letters
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Citations by publishers
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American Chemical Society (ACS)
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American Chemical Society (ACS)
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Springer Nature
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Multidisciplinary Digital Publishing Institute (MDPI)
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 6.25%
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American Institute of Physics (AIP)
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American Institute of Physics (AIP)
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Wiley
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Wiley
1 publication, 6.25%
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Royal Society of Chemistry (RSC)
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Royal Society of Chemistry (RSC)
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Walter de Gruyter
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Optical Society of America
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Pleiades Publishing
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1 publication, 6.25%
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IOP Publishing
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1 publication, 6.25%
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