Open Access
Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties
G I Dzhardimalieva
1, 2
,
Evgeniy V Vaganov
1
,
Valentina A Lesnichaya
1
,
Gulsara D Kugabaeva
1, 2
,
Publication type: Journal Article
Publication date: 2021-05-27
PubMed ID:
34072063
General Chemistry
Polymers and Plastics
Abstract
We report here our successful attempt to obtain self-healing supramolecular hydrogels with new metal-containing monomers (MCMs) with pendent 4-phenyl-2,2′:6′,2″-terpyridine metal complexes as reversible moieties by free radical copolymerization of MCMs with vinyl monomers, such as acrylic acid and acrylamide. The resulting metal-polymer hydrogels demonstrate a developed system of hydrogen, coordination and electron-complementary π–π stacking interactions, which play a critical role in achieving self-healing. Kinetic data show that the addition of a third metal-containing comonomer to the system decreases the initial polymerization rate, which is due to the specific effect of the metal group located in close proximity of the active center on the growth of radicals.
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9
Total citations:
9
Citations from 2024:
5
(55%)
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Baimuratova R. K. et al. Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties // Polymers. 2021. Vol. 13. No. 11. p. 1760.
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Baimuratova R. K., Dzhardimalieva G. I., Vaganov E. V., Lesnichaya V. A., Kugabaeva G. D., Kydralieva K. A., Zhinzhilo V. A., Uflyand I. E. Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties // Polymers. 2021. Vol. 13. No. 11. p. 1760.
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RIS
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TY - JOUR
DO - 10.3390/polym13111760
UR - https://doi.org/10.3390/polym13111760
TI - Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties
T2 - Polymers
AU - Baimuratova, Rose K
AU - Dzhardimalieva, G I
AU - Vaganov, Evgeniy V
AU - Lesnichaya, Valentina A
AU - Kugabaeva, Gulsara D
AU - Kydralieva, Kamila A
AU - Zhinzhilo, Vladimir A.
AU - Uflyand, Igor E.
PY - 2021
DA - 2021/05/27
PB - MDPI
SP - 1760
IS - 11
VL - 13
PMID - 34072063
SN - 2073-4360
ER -
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BibTex (up to 50 authors)
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@article{2021_Baimuratova,
author = {Rose K Baimuratova and G I Dzhardimalieva and Evgeniy V Vaganov and Valentina A Lesnichaya and Gulsara D Kugabaeva and Kamila A Kydralieva and Vladimir A. Zhinzhilo and Igor E. Uflyand},
title = {Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties},
journal = {Polymers},
year = {2021},
volume = {13},
publisher = {MDPI},
month = {may},
url = {https://doi.org/10.3390/polym13111760},
number = {11},
pages = {1760},
doi = {10.3390/polym13111760}
}
Cite this
MLA
Copy
Baimuratova, Rose K., et al. “Novel self-healing metallocopolymers with pendent 4-phenyl-2,2′:6′,2″-terpyridine ligand: Kinetic studies and mechanical properties.” Polymers, vol. 13, no. 11, May. 2021, p. 1760. https://doi.org/10.3390/polym13111760.