Open Access
Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials
D. M. Arkhipova
1, 2
,
Vadim V Ermolaev
2
,
Vasili Miluykov
2
,
Farida G Valeeva
2
,
Mikhail E. Minyaev
1
,
Publication type: Journal Article
Publication date: 2021-09-02
Renewable Energy, Sustainability and the Environment
Geography, Planning and Development
Management, Monitoring, Policy and Law
Abstract
A series of sterically hindered tri-tert-butyl(n-alkyl)phosphonium salts (n-CnH2n+1 with n = 1, 3, 5, 7, 9, 11, 13, 15, 17) was synthesized and systematically studied by 1H, 13C, 31P NMR spectroscopy, ESI-MS, single-crystal X-ray diffraction analysis and melting point measurement. Formation and stabilization palladium nanoparticles (PdNPs) were used to characterize the phosphonium ionic liquid (PIL) nanoscale interaction ability. The colloidal Pd in the PIL systems was described with TEM and DLS analyses and applied in the Suzuki cross-coupling reaction. The PILs were proven to be suitable stabilizers of PdNPs possessing high catalytic activity. The tri-tert-butyl(n-alkyl)phosphonium salts showed a complex nonlinear correlation of the structure–property relationship. The synthesized family of PILs has a broad variety of structural features, including hydrophobic and hydrophilic structures that are entirely expressed in the diversity of their properties
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13
Total citations:
13
Citations from 2024:
5
(38%)
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Arkhipova D. M. et al. Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials // Sustainability. 2021. Vol. 13. No. 17. p. 9862.
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Arkhipova D. M., Ermolaev V. V., Miluykov V., Valeeva F. G., Gaynanova G. A., Zakharova L. Ya., Minyaev M. E., Ananikov V. P. Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials // Sustainability. 2021. Vol. 13. No. 17. p. 9862.
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RIS
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TY - JOUR
DO - 10.3390/su13179862
UR - https://doi.org/10.3390/su13179862
TI - Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials
T2 - Sustainability
AU - Arkhipova, D. M.
AU - Ermolaev, Vadim V
AU - Miluykov, Vasili
AU - Valeeva, Farida G
AU - Gaynanova, Gulnara A
AU - Zakharova, Lucia Ya
AU - Minyaev, Mikhail E.
AU - Ananikov, Valentine P.
PY - 2021
DA - 2021/09/02
PB - MDPI
SP - 9862
IS - 17
VL - 13
SN - 2071-1050
ER -
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BibTex (up to 50 authors)
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@article{2021_Arkhipova,
author = {D. M. Arkhipova and Vadim V Ermolaev and Vasili Miluykov and Farida G Valeeva and Gulnara A Gaynanova and Lucia Ya Zakharova and Mikhail E. Minyaev and Valentine P. Ananikov},
title = {Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials},
journal = {Sustainability},
year = {2021},
volume = {13},
publisher = {MDPI},
month = {sep},
url = {https://doi.org/10.3390/su13179862},
number = {17},
pages = {9862},
doi = {10.3390/su13179862}
}
Cite this
MLA
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Arkhipova, D. M., et al. “Tri-tert-butyl(n-alkyl)phosphonium Ionic Liquids: Structure, Properties and Application as Hybrid Catalyst Nanomaterials.” Sustainability, vol. 13, no. 17, Sep. 2021, p. 9862. https://doi.org/10.3390/su13179862.