Open Access
Advanced Electronic Materials, volume 8, issue 7, pages 2101281
Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals
Fedorenko Roman S
1, 2
,
Kuevda Alexey V
1, 2, 3
,
Trukhanov Vasiliy A
1, 2
,
Konstantinov Vladislav G
1, 2
,
Sosorev Andrey Yu
2, 4
,
Sonina Alina A
5, 6
,
Kazantsev Maxim S
5
,
Surin Nikolay M.
1
,
Grigorian Souren
7
,
Borshchev Oleg V
1
,
Paraschuk Dmitry Yu.
1, 2
7
Department of Physics, University of Siegen Walter‐Flex‐Straße 3 D‐57072 Siegen Germany
|
Publication type: Journal Article
Publication date: 2022-03-11
Journal:
Advanced Electronic Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6.2
ISSN: 2199160X
Electronic, Optical and Magnetic Materials
Abstract
2D organic semiconductor single crystals comprising one or a few molecular layers of macroscopic lateral sizes are ideal materials for ultrathin, flexible, and transparent field‐effect devices—a platform for transistors and sensors. In recent years, these 2D materials have demonstrated high performance not inferior to their 3D counterparts. However, light emissive properties of 2D organic semiconductor single crystals have not yet been reported, and a combination of high charge‐carrier mobility and bright luminescence in one material is still a challenge for 2D organic optoelectronics. Emissive high‐mobility 2D organic semiconductor based on a [1]benzothieno[3,2‐b]benzothiophene (BTBT)‐derivative, 2,7‐bis(4‐decylphenyl)[1]benzothieno[3,2‐b][1]benzothiophene (DPBTBT), is presented here. DPBTBT molecules self‐organize in large‐area ultrathin single‐crystalline films consisting of one or a few molecular layers. These 2D single crystals perfectly suit as an active layer of organic field‐effect transistors in full accordance with Shockley's model and uniquely combine the high charge‐carrier mobility reaching 7.5 cm2 V–1 s–1 with prominent light emissive properties, which allow a demonstration of the first 2D organic light‐emitting transistor. The high charge‐carrier mobility and thermal stability of the crystalline phases, pronounced luminescence, and good shelf‐life stability suggest that emissive BTBT‐type molecules are a promising avenue for 2D organic optoelectronics.
Citations by journals
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1
2
3
|
|
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Materials Chemistry Frontiers
|
Materials Chemistry Frontiers
3 publications, 37.5%
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Vestnik Moskovskogo Universiteta Seriya 3 Fizika Astronomiya
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Vestnik Moskovskogo Universiteta Seriya 3 Fizika Astronomiya
2 publications, 25%
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Crystals
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Crystals
1 publication, 12.5%
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Dyes and Pigments
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Dyes and Pigments
1 publication, 12.5%
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Journal of Physical Chemistry C
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Journal of Physical Chemistry C
1 publication, 12.5%
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1
2
3
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Citations by publishers
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1
2
3
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Royal Society of Chemistry (RSC)
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Royal Society of Chemistry (RSC)
3 publications, 37.5%
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|
Moscow University Press
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Moscow University Press
2 publications, 25%
|
|
Multidisciplinary Digital Publishing Institute (MDPI)
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 12.5%
|
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Elsevier
|
Elsevier
1 publication, 12.5%
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American Chemical Society (ACS)
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American Chemical Society (ACS)
1 publication, 12.5%
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1
2
3
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Fedorenko R. S. et al. Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals // Advanced Electronic Materials. 2022. Vol. 8. No. 7. p. 2101281.
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Fedorenko R. S., Kuevda A. V., Trukhanov V. A., Konstantinov V. G., Sosorev A. Yu., Sonina A. A., Kazantsev M. S., Surin N. M., Grigorian S., Borshchev O. V., Ponomarenko S. A., Paraschuk D. Y. Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals // Advanced Electronic Materials. 2022. Vol. 8. No. 7. p. 2101281.
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TY - JOUR
DO - 10.1002/aelm.202101281
UR - https://doi.org/10.1002%2Faelm.202101281
TI - Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals
T2 - Advanced Electronic Materials
AU - Kuevda, Alexey V
AU - Trukhanov, Vasiliy A
AU - Konstantinov, Vladislav G
AU - Sosorev, Andrey Yu
AU - Sonina, Alina A
AU - Surin, Nikolay M.
AU - Ponomarenko, Sergey A
AU - Borshchev, Oleg V
AU - Kazantsev, Maxim S
AU - Grigorian, Souren
AU - Fedorenko, Roman S
AU - Paraschuk, Dmitry Yu.
PY - 2022
DA - 2022/03/11 00:00:00
PB - Wiley
SP - 2101281
IS - 7
VL - 8
SN - 2199-160X
ER -
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@article{2022_Fedorenko,
author = {Alexey V Kuevda and Vasiliy A Trukhanov and Vladislav G Konstantinov and Andrey Yu Sosorev and Alina A Sonina and Nikolay M. Surin and Sergey A Ponomarenko and Oleg V Borshchev and Maxim S Kazantsev and Souren Grigorian and Roman S Fedorenko and Dmitry Yu. Paraschuk},
title = {Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals},
journal = {Advanced Electronic Materials},
year = {2022},
volume = {8},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002%2Faelm.202101281},
number = {7},
pages = {2101281},
doi = {10.1002/aelm.202101281}
}
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MLA
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Fedorenko, Roman S., et al. “Luminescent High‐Mobility 2D Organic Semiconductor Single Crystals.” Advanced Electronic Materials, vol. 8, no. 7, Mar. 2022, p. 2101281. https://doi.org/10.1002%2Faelm.202101281.