Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights
Publication type: Journal Article
Publication date: 2008-05-16
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
18381724
General Chemistry
Catalysis
Abstract
Metal‐catalyzed cycloisomerization reactions of 1,n‐enynes have appeared as conceptually and chemically highly attractive processes as they contribute to the highly demanded search for atom economy and allow the discovery of new reactions. Since the pioneering studies with palladium by the research group of Barry Trost in the mid‐1980s, several other metals have been identified as excellent catalysts for the rearrangement of enyne skeletons. Moreover, the behavior of 1,n‐enynes may be influenced by other functional groups such as alcohols, aldehydes, ethers, alkenes, or alkynes, thus enhancing the molecular complexity of the synthesized products. Apart from the intrinsic rearrangements of 1,n‐enynes, several tandem reactions incorporating intramolecular trapping agents or intermolecular partners have been discovered. This Review aims to highlight the main contributions in this field of catalysis and to propose and comment on the mechanistic insights of the recent discoveries.
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Michelet V., Toullec P., Genêt J. Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights // Angewandte Chemie - International Edition. 2008. Vol. 47. No. 23. pp. 4268-4315.
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Michelet V., Toullec P., Genêt J. Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights // Angewandte Chemie - International Edition. 2008. Vol. 47. No. 23. pp. 4268-4315.
Cite this
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TY - JOUR
DO - 10.1002/anie.200701589
UR - https://onlinelibrary.wiley.com/doi/10.1002/anie.200701589
TI - Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights
T2 - Angewandte Chemie - International Edition
AU - Michelet, Véronique
AU - Toullec, Patrick
AU - Genêt, Jean-Pierre
PY - 2008
DA - 2008/05/16
PB - Wiley
SP - 4268-4315
IS - 23
VL - 47
PMID - 18381724
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
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@article{2008_Michelet,
author = {Véronique Michelet and Patrick Toullec and Jean-Pierre Genêt},
title = {Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights},
journal = {Angewandte Chemie - International Edition},
year = {2008},
volume = {47},
publisher = {Wiley},
month = {may},
url = {https://onlinelibrary.wiley.com/doi/10.1002/anie.200701589},
number = {23},
pages = {4268--4315},
doi = {10.1002/anie.200701589}
}
Cite this
MLA
Copy
Michelet, Véronique, et al. “Cycloisomerization of 1,n‐Enynes: Challenging Metal‐Catalyzed Rearrangements and Mechanistic Insights.” Angewandte Chemie - International Edition, vol. 47, no. 23, May. 2008, pp. 4268-4315. https://onlinelibrary.wiley.com/doi/10.1002/anie.200701589.