Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination.
Publication type: Journal Article
Publication date: 2018-04-23
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
29603565
General Chemistry
Catalysis
Abstract
Electrocatalysis has been identified as a powerful strategy for organometallic catalysis, and yet electrocatalytic C-H activation is restricted to strongly N-coordinating directing groups. The first example of electrocatalytic C-H activation by weak O-coordination is presented, in which a versatile ruthenium(II) carboxylate catalyst enables electrooxidative C-H/O-H functionalization for alkyne annulations in the absence of metal oxidants; thereby exploiting sustainable electricity as the sole oxidant. Mechanistic insights provide strong support for a facile organometallic C-H ruthenation and an effective electrochemical reoxidation of the key ruthenium(0) intermediate.
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Metrics
196
Total citations:
196
Citations from 2024:
20
(10.2%)
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GOST
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Qiu Y. et al. Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination. // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 20. pp. 5818-5822.
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Qiu Y., Tian C., Massignan L., Rogge T., Ackermann L. Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination. // Angewandte Chemie - International Edition. 2018. Vol. 57. No. 20. pp. 5818-5822.
Cite this
RIS
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TY - JOUR
DO - 10.1002/anie.201802748
UR - https://doi.org/10.1002/anie.201802748
TI - Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination.
T2 - Angewandte Chemie - International Edition
AU - Qiu, Youai
AU - Tian, Cong
AU - Massignan, Leonardo
AU - Rogge, Torben
AU - Ackermann, Lutz
PY - 2018
DA - 2018/04/23
PB - Wiley
SP - 5818-5822
IS - 20
VL - 57
PMID - 29603565
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
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@article{2018_Qiu,
author = {Youai Qiu and Cong Tian and Leonardo Massignan and Torben Rogge and Lutz Ackermann},
title = {Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination.},
journal = {Angewandte Chemie - International Edition},
year = {2018},
volume = {57},
publisher = {Wiley},
month = {apr},
url = {https://doi.org/10.1002/anie.201802748},
number = {20},
pages = {5818--5822},
doi = {10.1002/anie.201802748}
}
Cite this
MLA
Copy
Qiu, Youai, et al. “Electrooxidative Ruthenium-Catalyzed C-H/O-H Annulation by Weak O-Coordination..” Angewandte Chemie - International Edition, vol. 57, no. 20, Apr. 2018, pp. 5818-5822. https://doi.org/10.1002/anie.201802748.