Chemistry - A European Journal

, том 21 , издание 46 , страницы 16344-16348

General Route to Cyclobutadiene Rhodium Complexes

Тип публикации: Journal Article

Дата публикации: 2015-09-21

Wiley

Chemistry - A European Journal

scimago Q1

wos Q2

white level БС1

SJR: 0.981

CiteScore: 6.7

Impact factor: 3.7

ISSN: 09476539, 15213765

DOI: 10.1002/chem.201503270

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PubMed ID: 26387565

General Chemistry

Catalysis

Organic Chemistry

Краткое описание

Cyclobutadiene rhodium complexes bear high potential for applications in organometallic synthesis and catalysis. We have found that the cyclobutadiene complexes with substitutionally labile p‐xylene ligands [(C₄R₄)Rh(p‐xylene)]⁺ can be synthesized in one step from the commercially available bis(ethylene) complex [{(C₂H₄)₂RhCl}₂], p‐xylene, and internal alkynes. The replacement of p‐xylene by various ligands provides a general access to other [(C₄R₄)Rh] compounds, such as [(C₄R₄)RhCl]_x, [(C₄R₄)RhL₃]⁺, [(C₄R₄)Rh(C₅H₅)], and [(C₄R₄)Rh(arene)]⁺. Complex [(C₄Et₄)Rh(p‐xylene)]⁺ also catalyzes an unusual cycloisomerization of a 1,11‐dien‐6‐yne into a bicyclic diene.

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Perekalin D. S. et al. General Route to Cyclobutadiene Rhodium Complexes // Chemistry - A European Journal. 2015. Vol. 21. No. 46. pp. 16344-16348.

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Perekalin D. S., Shvydkiy N. V., Nelyubina Y. V., Kudinov A. R. General Route to Cyclobutadiene Rhodium Complexes // Chemistry - A European Journal. 2015. Vol. 21. No. 46. pp. 16344-16348.

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TY - JOUR

DO - 10.1002/chem.201503270

UR - https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270

TI - General Route to Cyclobutadiene Rhodium Complexes

T2 - Chemistry - A European Journal

AU - Perekalin, Dmitry S

AU - Shvydkiy, Nikita V

AU - Nelyubina, Yulia V.

AU - Kudinov, Alexander R

PY - 2015

DA - 2015/09/21

PB - Wiley

SP - 16344-16348

IS - 46

VL - 21

PMID - 26387565

SN - 0947-6539

SN - 1521-3765

ER -

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@article{2015_Perekalin,

author = {Dmitry S Perekalin and Nikita V Shvydkiy and Yulia V. Nelyubina and Alexander R Kudinov},

title = {General Route to Cyclobutadiene Rhodium Complexes},

journal = {Chemistry - A European Journal},

year = {2015},

volume = {21},

publisher = {Wiley},

month = {sep},

url = {https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270},

number = {46},

pages = {16344--16348},

doi = {10.1002/chem.201503270}

}

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Perekalin, Dmitry S., et al. “General Route to Cyclobutadiene Rhodium Complexes.” Chemistry - A European Journal, vol. 21, no. 46, Sep. 2015, pp. 16344-16348. https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270.

Ошибка в публикации?

Издатель

Wiley

Журнал

Chemistry - A European Journal

scimago Q1

wos Q2

white level БС1

SJR

0.981

CiteScore

6.7

Impact factor

3.7

ISSN

09476539 (Print)

15213765 (Electronic)

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