Green nanocomposite gels based on binary network of sodium alginate and percolating halloysite clay nanotubes for 3D printing
Publication type: Journal Article
Publication date: 2022-04-01
scimago Q1
wos Q1
SJR: 2.004
CiteScore: 24.0
Impact factor: 12.5
ISSN: 01448617, 18791344
PubMed ID:
35123742
Materials Chemistry
Organic Chemistry
Polymers and Plastics
Abstract
Alginate hydrogels with embedded rigid percolating network of halloysite clay nanotubes were evaluated as a novel ink for 3D printing. Hydrophilic alginate macromolecules adsorbing on halloysite stabilize the network of the nanotubes and form their own network of interlaced polymer chains. The effect of halloysite content on the structure and properties of the hydrogels was studied by rheometry, thermogravimetric analysis, FTIR-spectroscopy, dynamic light scattering, transmission electron microscopy, and 3D cryo-electron microscopy. Hydrogels demonstrate a very pronounced shear-thinning at extrusion and rather quick viscosity recovery after extrusion assigned to rapid rearrangement of the network structure promoted by mobile alginate chains. Even at low volume fractions (up to 0.054) the nanotubes reinforce the hydrogel increasing its storage modulus up to 650 Pa and inducing the appearance of yield stress. These properties make the alginate/halloysite hydrogels promising for the application in 3D printing for fabrication of green and sustainable nanocomposite materials made from natural components.
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Total citations:
29
Citations from 2025:
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(20.69%)
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Glukhova S. A. et al. Green nanocomposite gels based on binary network of sodium alginate and percolating halloysite clay nanotubes for 3D printing // Carbohydrate Polymers. 2022. Vol. 282. p. 119106.
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Glukhova S. A., Molchanov V. S., Chesnokov Y., Lokshin B., Kharitonova E., Philippova O. Green nanocomposite gels based on binary network of sodium alginate and percolating halloysite clay nanotubes for 3D printing // Carbohydrate Polymers. 2022. Vol. 282. p. 119106.
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TY - JOUR
DO - 10.1016/j.carbpol.2022.119106
UR - https://doi.org/10.1016/j.carbpol.2022.119106
TI - Green nanocomposite gels based on binary network of sodium alginate and percolating halloysite clay nanotubes for 3D printing
T2 - Carbohydrate Polymers
AU - Glukhova, Svetlana A.
AU - Molchanov, Vyacheslav S
AU - Chesnokov, Yu.M.
AU - Lokshin, Boris
AU - Kharitonova, E.
AU - Philippova, O.E.
PY - 2022
DA - 2022/04/01
PB - Elsevier
SP - 119106
VL - 282
PMID - 35123742
SN - 0144-8617
SN - 1879-1344
ER -
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@article{2022_Glukhova,
author = {Svetlana A. Glukhova and Vyacheslav S Molchanov and Yu.M. Chesnokov and Boris Lokshin and E. Kharitonova and O.E. Philippova},
title = {Green nanocomposite gels based on binary network of sodium alginate and percolating halloysite clay nanotubes for 3D printing},
journal = {Carbohydrate Polymers},
year = {2022},
volume = {282},
publisher = {Elsevier},
month = {apr},
url = {https://doi.org/10.1016/j.carbpol.2022.119106},
pages = {119106},
doi = {10.1016/j.carbpol.2022.119106}
}