volume 696 issue 1 pages 400-405

NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction

Publication typeJournal Article
Publication date2011-01-01
scimago Q3
wos Q2
SJR0.385
CiteScore4.1
Impact factor2.4
ISSN0022328X, 18728561
Materials Chemistry
Organic Chemistry
Biochemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Abstract In the present study we have analyzed the nature of palladium complexes in the catalytic system for selective carbon–sulfur bond formation via the addition of S–S and S–H bonds to alkynes. For the first time the mononuclear and dinuclear palladium complexes were clearly detected by DOSY NMR under the catalytic conditions. It was demonstrated that the concentration of these palladium complexes strongly depends on the amount of phosphine ligand available under reaction conditions.
Found 
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Ananikov V. P. et al. NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction // Journal of Organometallic Chemistry. 2011. Vol. 696. No. 1. pp. 400-405.
GOST all authors (up to 50) Copy
Ananikov V. P., Kachala V. V., S. Zalesskiy S., Beletskaya I. P. NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction // Journal of Organometallic Chemistry. 2011. Vol. 696. No. 1. pp. 400-405.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1016/j.jorganchem.2010.10.012
UR - https://doi.org/10.1016/j.jorganchem.2010.10.012
TI - NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction
T2 - Journal of Organometallic Chemistry
AU - Ananikov, Valentine P.
AU - Kachala, Vadim V.
AU - S. Zalesskiy, Sergey
AU - Beletskaya, Irina P.
PY - 2011
DA - 2011/01/01
PB - Elsevier
SP - 400-405
IS - 1
VL - 696
SN - 0022-328X
SN - 1872-8561
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2011_Ananikov,
author = {Valentine P. Ananikov and Vadim V. Kachala and Sergey S. Zalesskiy and Irina P. Beletskaya},
title = {NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction},
journal = {Journal of Organometallic Chemistry},
year = {2011},
volume = {696},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.jorganchem.2010.10.012},
number = {1},
pages = {400--405},
doi = {10.1016/j.jorganchem.2010.10.012}
}
MLA
Cite this
MLA Copy
Ananikov, Valentine P., et al. “NMR approach for the identification of dinuclear and mononuclear complexes: The first detection of [Pd(SPh)2(PPh3)2] and [Pd2(SPh)4(PPh3)2] - The intermediate complexes in the catalytic carbon-sulfur bond formation reaction.” Journal of Organometallic Chemistry, vol. 696, no. 1, Jan. 2011, pp. 400-405. https://doi.org/10.1016/j.jorganchem.2010.10.012.