Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene
Pavel Markov
1
,
Galina N Baeva
1
,
Publication type: Journal Article
Publication date: 2020-07-01
scimago Q3
wos Q3
SJR: 0.305
CiteScore: 3.0
Impact factor: 1.7
ISSN: 09599436, 1364551X
General Chemistry
Abstract
Novel one-pot synthesis of trans-stilbene comprises hydrogenation of diphenylacetylene into cis-stilbene followed by its hydroisomerization, over the catalyst being intermetallic PdxIny/Al2O3 system with isolated single-atom Pd1 sites. The hydroisomerization rate in the process is comparable or exceeds the over-hydrogenation into 1,2-diphenylethane thus providing 76% yield of trans-stilbene in the case of Pd2In3/Al2O3 catalyst. This result presumably stems from the formation of ordered single-atom Pd1 sites with favorable hydroisomerization ability on the surface of PdxIny catalysts.
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Total citations:
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Citations from 2024:
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(25%)
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Markov P. et al. Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene // Mendeleev Communications. 2020. Vol. 30. No. 4. pp. 468-471.
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Markov P., Smirnova N. V., Baeva G. N., Bukhtiyarov A. V., Mashkovsky I. S., Stakheev A. Yu. Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene // Mendeleev Communications. 2020. Vol. 30. No. 4. pp. 468-471.
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TY - JOUR
DO - 10.1016/j.mencom.2020.07.020
UR - https://doi.org/10.1016/j.mencom.2020.07.020
TI - Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene
T2 - Mendeleev Communications
AU - Markov, Pavel
AU - Smirnova, Nadezhda V.
AU - Baeva, Galina N
AU - Bukhtiyarov, Andrey V
AU - Mashkovsky, Igor S
AU - Stakheev, Alexander Yu
PY - 2020
DA - 2020/07/01
PB - OOO Zhurnal "Mendeleevskie Soobshcheniya"
SP - 468-471
IS - 4
VL - 30
SN - 0959-9436
SN - 1364-551X
ER -
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BibTex (up to 50 authors)
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@article{2020_Markov,
author = {Pavel Markov and Nadezhda V. Smirnova and Galina N Baeva and Andrey V Bukhtiyarov and Igor S Mashkovsky and Alexander Yu Stakheev},
title = {Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene},
journal = {Mendeleev Communications},
year = {2020},
volume = {30},
publisher = {OOO Zhurnal "Mendeleevskie Soobshcheniya"},
month = {jul},
url = {https://doi.org/10.1016/j.mencom.2020.07.020},
number = {4},
pages = {468--471},
doi = {10.1016/j.mencom.2020.07.020}
}
Cite this
MLA
Copy
Markov, Pavel, et al. “Intermetallic Pd In /Al2O3 catalysts with isolated single-atom Pd sites for one-pot hydrogenation of diphenylacetylene into trans-stilbene.” Mendeleev Communications, vol. 30, no. 4, Jul. 2020, pp. 468-471. https://doi.org/10.1016/j.mencom.2020.07.020.