Deep-red phosphorescent organic–inorganic hybrid Mn(II) complexes based on 2-(diphenylphosphoryl)-N,N-diethylacetamide ligand
Publication type: Journal Article
Publication date: 2018-07-01
scimago Q3
wos Q2
SJR: 0.396
CiteScore: 4.9
Impact factor: 2.6
ISSN: 02775387, 18733719
Materials Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Two unprecedented organic–inorganic hybrid complexes, [Mn(L)3]MnCl4 (1) and [Mn(L)3]MnBr4 (2), have been synthesized in 88–92% yields via reaction of Mn(II) halides with Ph2P(O)CH2C(O)NEt2 (L) in a 3:2 M ratio. X-ray diffraction analysis of 2 reveals that the metal ion of the [Mn(L)3]2+ cation has an octahedral geometry, while the [MnBr4]2− anion contains tetrahedrally coordinated Mn(II). At ambient temperature, the solid complexes 1 and 2 exhibit bright deep-red phosphorescence ( λ max em = 660 and 670 nm) with the lifetimes of 3–3.7 ms and photoluminescence quantum yields of 6% and 27%, respectively.
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Total citations:
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(11.54%)
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Artem'ev A. V. et al. Deep-red phosphorescent organic–inorganic hybrid Mn(II) complexes based on 2-(diphenylphosphoryl)-N,N-diethylacetamide ligand // Polyhedron. 2018. Vol. 148. pp. 184-188.
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Artem'ev A. V., Berezin A. S., Brel V. K., Morgalyuk V. P., Samsonenko D. G. Deep-red phosphorescent organic–inorganic hybrid Mn(II) complexes based on 2-(diphenylphosphoryl)-N,N-diethylacetamide ligand // Polyhedron. 2018. Vol. 148. pp. 184-188.
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TY - JOUR
DO - 10.1016/j.poly.2018.04.012
UR - https://doi.org/10.1016/j.poly.2018.04.012
TI - Deep-red phosphorescent organic–inorganic hybrid Mn(II) complexes based on 2-(diphenylphosphoryl)-N,N-diethylacetamide ligand
T2 - Polyhedron
AU - Artem'ev, Alexander V.
AU - Berezin, Alexei S
AU - Brel, Valery K.
AU - Morgalyuk, V. P.
AU - Samsonenko, Denis G.
PY - 2018
DA - 2018/07/01
PB - Elsevier
SP - 184-188
VL - 148
SN - 0277-5387
SN - 1873-3719
ER -
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@article{2018_Artem'ev,
author = {Alexander V. Artem'ev and Alexei S Berezin and Valery K. Brel and V. P. Morgalyuk and Denis G. Samsonenko},
title = {Deep-red phosphorescent organic–inorganic hybrid Mn(II) complexes based on 2-(diphenylphosphoryl)-N,N-diethylacetamide ligand},
journal = {Polyhedron},
year = {2018},
volume = {148},
publisher = {Elsevier},
month = {jul},
url = {https://doi.org/10.1016/j.poly.2018.04.012},
pages = {184--188},
doi = {10.1016/j.poly.2018.04.012}
}