, volume 19 , issue 20 , pages 5657-5660

Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination

Pavel N Kolesnikov ¹

Karim M Muratov ^{1, 2}

Denis Chusov ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

A.N. Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences, Vavilova St. 28, Moscow 119991, Russian Federation |

Dmitry Mendeleev University of Chemical Technology of Russia, Miusskaya sq. 9, Moscow 125047, Russian Federation |

Publication type: Journal Article

Publication date: 2017-09-29

American Chemical Society (ACS)

Organic Letters

scimago Q1

wos Q1

SJR: 1.235

CiteScore: 8.7

Impact factor: 5.0

ISSN: 15237060, 15237052

DOI: 10.1021/acs.orglett.7b02821

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PubMed ID: 28961011

Organic Chemistry

Biochemistry

Physical and Theoretical Chemistry

Abstract

Rh-catalyzed one-step reductive amidation of aldehydes has been developed. The protocol does not require an external hydrogen source and employs carbon monoxide as a deoxygenative agent. The direction of the reaction can be altered simply by changing the solvent: reaction in THF leads to amides, whereas methanol favors formation of tertiary amines.

Found

8 citations

Chusov Denis

DSc in Chemistry, professor

99 publications, 2 395 citations, 35 reviews

h-index: 25

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Asymmetric metal complex catalysis

2 citations

Loginov Dmitry

🥼

DSc in Chemistry

126 publications, 1 795 citations, 36 reviews

h-index: 25

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Catalysis

Coordination Chemistry

Organic Chemistry

Organic synthesis

Organometallic Chemistry

Photonics

1 citation

Khrustalev Victor

DSc in Chemistry, professor, professor of the Russian Academy of Sciences

326 publications, 4 094 citations, 4 reviews

h-index: 30

N.D. Zelinsky Institute of Organic Chemistry of the Russian Academy of Sciences

Peoples' Friendship University of Russia

1 citation

Shubina Elena

DSc in Chemistry, professor

264 publications, 5 882 citations, 16 reviews

h-index: 38

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Molecular spectroscopy

1 citation

Nelyubina Yulia

🤝

DSc in Chemistry

506 publications, 7 606 citations, 1 review

h-index: 38

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Moscow Institute of Physics and Technology

Metal-organic frameworks

Quantum technologies

Sensors

1 citation

Bilyachenko Alexey

🥼 🤝

DSc in Chemistry

88 publications, 2 089 citations, 13 reviews

h-index: 28

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Peoples' Friendship University of Russia

1 citation

Perekalin Dmitry

🥼

DSc in Chemistry

121 publications, 1 974 citations, 35 reviews

h-index: 25

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Asymmetric metal complex catalysis

Catalysis

Organometallic Chemistry

Photochemistry

1 citation

Kharitonov Vladimir

23 publications, 253 citations

h-index: 10

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Catalysis

Density functional theory (DFT)

Organic Chemistry

Organometallic Chemistry

1 citation

Arsenov Mikhail

13 publications, 125 citations

h-index: 7

A.N.Nesmeyanov Institute of Organoelement Compounds of the Russian Academy of Sciences

Research interests

Asymmetric metal complex catalysis

Catalysis

Organic Chemistry

Organoelement chemistry

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Kolesnikov P. N. et al. Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination // Organic Letters. 2017. Vol. 19. No. 20. pp. 5657-5660.

GOST all authors (up to 50) Copy

Kolesnikov P. N., Muratov K. M., Chusov D. Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination // Organic Letters. 2017. Vol. 19. No. 20. pp. 5657-5660.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.orglett.7b02821

UR - https://doi.org/10.1021/acs.orglett.7b02821

TI - Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination

T2 - Organic Letters

AU - Kolesnikov, Pavel N

AU - Muratov, Karim M

AU - Chusov, Denis

PY - 2017

DA - 2017/09/29

PB - American Chemical Society (ACS)

SP - 5657-5660

IS - 20

VL - 19

PMID - 28961011

SN - 1523-7060

SN - 1523-7052

ER -

BibTex |

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BibTex (up to 50 authors) Copy

@article{2017_Kolesnikov,

author = {Pavel N Kolesnikov and Karim M Muratov and Denis Chusov},

title = {Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination},

journal = {Organic Letters},

year = {2017},

volume = {19},

publisher = {American Chemical Society (ACS)},

month = {sep},

url = {https://doi.org/10.1021/acs.orglett.7b02821},

number = {20},

pages = {5657--5660},

doi = {10.1021/acs.orglett.7b02821}

}

MLA

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Kolesnikov, Pavel N., et al. “Dichotomy of Atom-Economical Hydrogen-Free Reductive Amidation vs Exhaustive Reductive Amination.” Organic Letters, vol. 19, no. 20, Sep. 2017, pp. 5657-5660. https://doi.org/10.1021/acs.orglett.7b02821.