volume 137 issue 31 pages 9792-9795

A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior

Publication typeJournal Article
Publication date2015-07-28
scimago Q1
wos Q1
SJR5.554
CiteScore22.5
Impact factor15.6
ISSN00027863, 15205126
PubMed ID:  26199996
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Single-molecule magnets (SMMs) with one transition-metal ion often rely on unusual geometry as a source of magnetically anisotropic ground state. Here we report a cobalt(II) cage complex with a trigonal prism geometry showing single ion magnet behavior with very high Orbach relaxation barrier of 152 cm(-1). This, to our knowledge, is the largest reported relaxation barrier for a cobalt-based mononuclear SMM. The trigonal prismatic coordination provided by the macrocyclic ligand gives intrinsically more stable molecular species than previously reported SMMs, thus making this type of cage complexes more amendable to possible functionalization that will boost their magnetic anisotropy even further.
Found 
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GOST Copy
Novikov V. V. et al. A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior // Journal of the American Chemical Society. 2015. Vol. 137. No. 31. pp. 9792-9795.
GOST all authors (up to 50) Copy
Novikov V. V., Pavlov A., Nelyubina Y. V., Boulon M., Varzatskii O. A., Voloshin Y. Z., Winpenny R. E. P. A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior // Journal of the American Chemical Society. 2015. Vol. 137. No. 31. pp. 9792-9795.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/jacs.5b05739
UR - https://doi.org/10.1021/jacs.5b05739
TI - A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior
T2 - Journal of the American Chemical Society
AU - Novikov, Valentin V
AU - Pavlov, Alexander
AU - Nelyubina, Yulia V.
AU - Boulon, M.-E.
AU - Varzatskii, Oleg A
AU - Voloshin, Yan Z.
AU - Winpenny, Richard E. P.
PY - 2015
DA - 2015/07/28
PB - American Chemical Society (ACS)
SP - 9792-9795
IS - 31
VL - 137
PMID - 26199996
SN - 0002-7863
SN - 1520-5126
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2015_Novikov,
author = {Valentin V Novikov and Alexander Pavlov and Yulia V. Nelyubina and M.-E. Boulon and Oleg A Varzatskii and Yan Z. Voloshin and Richard E. P. Winpenny},
title = {A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior},
journal = {Journal of the American Chemical Society},
year = {2015},
volume = {137},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/jacs.5b05739},
number = {31},
pages = {9792--9795},
doi = {10.1021/jacs.5b05739}
}
MLA
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MLA Copy
Novikov, Valentin V., et al. “A Trigonal Prismatic Mononuclear Cobalt(II) Complex Showing Single-Molecule Magnet Behavior.” Journal of the American Chemical Society, vol. 137, no. 31, Jul. 2015, pp. 9792-9795. https://doi.org/10.1021/jacs.5b05739.