Associating Polymers: Equilibrium and Linear Viscoelasticity
Publication type: Journal Article
Publication date: 1995-02-01
scimago Q1
wos Q1
SJR: 1.352
CiteScore: 9.0
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
A theory for the equilibrium and dynamic properties of a solution of telechelic polymers in the limit of high aggregation number is presented. It is shown that (1) the micelles formed by telechelic chains (flowers) in a dilute solution strongly attract each other, (2) at some concentration φ* the flowers form a reversible gel where they are connected by multiple bridges, (3) the dynamics of individual micelles in the gel is governed by the bridge/loop exchange rate and by the effective barrier associated with the hopping of a micelle to a new position ; this barrier is determined by the energy associated to a deformation/compression of a micelle, (4) the viscosity is changing exponentially in the region φ > φ* (it is increasing in the vicinity of φ*) ; however, it can decrease (with φ) in a limited concentration range above φ*.
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427
Total citations:
427
Citations from 2024:
11
(2.58%)
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GOST
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Semenov A. N., JOANNY J., Khokhlov A. R. Associating Polymers: Equilibrium and Linear Viscoelasticity // Macromolecules. 1995. Vol. 28. No. 4. pp. 1066-1075.
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Semenov A. N., JOANNY J., Khokhlov A. R. Associating Polymers: Equilibrium and Linear Viscoelasticity // Macromolecules. 1995. Vol. 28. No. 4. pp. 1066-1075.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ma00108a038
UR - https://doi.org/10.1021/ma00108a038
TI - Associating Polymers: Equilibrium and Linear Viscoelasticity
T2 - Macromolecules
AU - Semenov, A. N.
AU - JOANNY, J.-F.
AU - Khokhlov, A R
PY - 1995
DA - 1995/02/01
PB - American Chemical Society (ACS)
SP - 1066-1075
IS - 4
VL - 28
SN - 0024-9297
SN - 1520-5835
ER -
Cite this
BibTex (up to 50 authors)
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@article{1995_Semenov,
author = {A. N. Semenov and J.-F. JOANNY and A R Khokhlov},
title = {Associating Polymers: Equilibrium and Linear Viscoelasticity},
journal = {Macromolecules},
year = {1995},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/ma00108a038},
number = {4},
pages = {1066--1075},
doi = {10.1021/ma00108a038}
}
Cite this
MLA
Copy
Semenov, A. N., et al. “Associating Polymers: Equilibrium and Linear Viscoelasticity.” Macromolecules, vol. 28, no. 4, Feb. 1995, pp. 1066-1075. https://doi.org/10.1021/ma00108a038.
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