Macromolecules, volume 47, issue 15, pages 5400-5408
Study of the mechanisms of filler reinforcement in elastomer nanocomposites
1
2
Institute
for Advanced Energy Related Nanomaterials, University of Ulm, Albert-Einstein-Allee
47, Ulm D-89069, Germany
|
Publication type: Journal Article
Publication date: 2014-07-14
Journal:
Macromolecules
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 5.5
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
We performed a large-scale dissipative dynamics simulation to study the structural changes in unfilled and filled elastomers during uniaxial deformation, which helped to shed some light on the underlying reasons of filler reinforcement in rubber nanocomposites. Equilibrium stress–stain curves for different cross-linker concentrations and filler content were obtained, and their features were compared to the experimental data. Dependences of segmental orientation on deformation and true stress were studied; these dependences are discussed in the light of theoretical predictions and available experimental data. The structural changes in the deformed state were studied as well, namely, the dependences of mean end-to-end distance on the subchain length. For the filled elastomers it was found that in the matrix there are several sets of subchains with distinct properties. Part of the subchains which are not connected to the filler particles are deformed slightly more than in the unfilled matrix; the subchains c...
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Gavrilov A. A. et al. Study of the mechanisms of filler reinforcement in elastomer nanocomposites // Macromolecules. 2014. Vol. 47. No. 15. pp. 5400-5408.
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Gavrilov A. A., Chertovich A. V., Khalatur P. G., Khokhlov A. R. Study of the mechanisms of filler reinforcement in elastomer nanocomposites // Macromolecules. 2014. Vol. 47. No. 15. pp. 5400-5408.
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TY - JOUR
DO - 10.1021/ma500947g
UR - https://doi.org/10.1021%2Fma500947g
TI - Study of the mechanisms of filler reinforcement in elastomer nanocomposites
T2 - Macromolecules
AU - Gavrilov, Alexey A.
AU - Chertovich, Alexander V.
AU - Khalatur, Pavel G
AU - Khokhlov, Alexei R.
PY - 2014
DA - 2014/07/14 00:00:00
PB - American Chemical Society (ACS)
SP - 5400-5408
IS - 15
VL - 47
SN - 0024-9297
SN - 1520-5835
ER -
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@article{2014_Gavrilov,
author = {Alexey A. Gavrilov and Alexander V. Chertovich and Pavel G Khalatur and Alexei R. Khokhlov},
title = {Study of the mechanisms of filler reinforcement in elastomer nanocomposites},
journal = {Macromolecules},
year = {2014},
volume = {47},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021%2Fma500947g},
number = {15},
pages = {5400--5408},
doi = {10.1021/ma500947g}
}
Cite this
MLA
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Gavrilov, Alexey A., et al. “Study of the mechanisms of filler reinforcement in elastomer nanocomposites.” Macromolecules, vol. 47, no. 15, Jul. 2014, pp. 5400-5408. https://doi.org/10.1021%2Fma500947g.