volume 41 issue 20 pages 7722-7728

Self-organization in solutions of stiff-chain amphiphilic macromolecules

Publication typeJournal Article
Publication date2008-09-24
scimago Q1
wos Q1
SJR1.352
CiteScore9.0
Impact factor5.2
ISSN00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
Conformational properties of amphiphilic stiff-chain macromolecules in concentrated solutions in poor solvent have been studied via computer modeling. We have found that the conformational state of macromolecules in such systems depends on the macromolecular stiffness and on the way the solution has been prepared. Thus, if the concentration of globules increased from a very diluted solution, the globules remain stable, independent of the macromolecular stiffness, and do not aggregate even in concentrated solutions. On the other hand, if the solvent quality is gradually decreased in a solution with a concentration much larger than that of a semidilute solution, then relatively flexible chains form separate globules, whereas semirigid macromolecules tend to aggregate and form braid-like conformations. The results obtained agree with the published experimental data and can be used for directed synthesis of macromolecules modeling the behavior of biopolymers.
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GOST |
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GOST Copy
Vasilevskaya V. V. et al. Self-organization in solutions of stiff-chain amphiphilic macromolecules // Macromolecules. 2008. Vol. 41. No. 20. pp. 7722-7728.
GOST all authors (up to 50) Copy
Vasilevskaya V. V., Markov V., ten Brinke G., Khokhlov A. R. Self-organization in solutions of stiff-chain amphiphilic macromolecules // Macromolecules. 2008. Vol. 41. No. 20. pp. 7722-7728.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/ma800465j
UR - https://doi.org/10.1021/ma800465j
TI - Self-organization in solutions of stiff-chain amphiphilic macromolecules
T2 - Macromolecules
AU - Vasilevskaya, V. V.
AU - Markov, V.A
AU - ten Brinke, G.
AU - Khokhlov, Alexei R.
PY - 2008
DA - 2008/09/24
PB - American Chemical Society (ACS)
SP - 7722-7728
IS - 20
VL - 41
SN - 0024-9297
SN - 1520-5835
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2008_Vasilevskaya,
author = {V. V. Vasilevskaya and V.A Markov and G. ten Brinke and Alexei R. Khokhlov},
title = {Self-organization in solutions of stiff-chain amphiphilic macromolecules},
journal = {Macromolecules},
year = {2008},
volume = {41},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/ma800465j},
number = {20},
pages = {7722--7728},
doi = {10.1021/ma800465j}
}
MLA
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MLA Copy
Vasilevskaya, V. V., et al. “Self-organization in solutions of stiff-chain amphiphilic macromolecules.” Macromolecules, vol. 41, no. 20, Sep. 2008, pp. 7722-7728. https://doi.org/10.1021/ma800465j.