Open Access
Nano Letters, volume 14, issue 2, pages 676-681
Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond
2
Publication type: Journal Article
Publication date: 2014-01-27
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
We explore how a few-layer graphene can undergo phase transformation into thin diamond film under reduced or no pressure, if the process is facilitated by hydrogenation of the surfaces. Such a "chemically induced phase transition" is inherently nanoscale phenomenon, when the surface conditions directly affect thermodynamics, and the transition pressure depends greatly on film thickness. For the first time we obtain, by ab initio computations of the Gibbs free energy, a phase diagram (P, T, h) of quasi-two-dimensional carbon-diamond film versus multilayered graphene. It describes accurately the role of film thickness h and shows the feasibility of creating novel quasi-two-dimensional materials. Further, the role of finite diameter of graphene flakes and possible formation of the diamond films with the (110) surface are described as well.
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Kvashnin A. G. et al. Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond // Nano Letters. 2014. Vol. 14. No. 2. pp. 676-681.
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Kvashnin A. G., Chernozatonskii L. A., Yakobson B. I., Sorokin P. B. Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond // Nano Letters. 2014. Vol. 14. No. 2. pp. 676-681.
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TY - JOUR
DO - 10.1021/nl403938g
UR - https://doi.org/10.1021/nl403938g
TI - Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond
T2 - Nano Letters
AU - Kvashnin, Alexander G.
AU - Chernozatonskii, Leonid A.
AU - Yakobson, Boris I.
AU - Sorokin, Pavel B.
PY - 2014
DA - 2014/01/27
PB - American Chemical Society (ACS)
SP - 676-681
IS - 2
VL - 14
SN - 1530-6984
SN - 1530-6992
ER -
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BibTex (up to 50 authors)
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@article{2014_Kvashnin,
author = {Alexander G. Kvashnin and Leonid A. Chernozatonskii and Boris I. Yakobson and Pavel B. Sorokin},
title = {Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond},
journal = {Nano Letters},
year = {2014},
volume = {14},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/nl403938g},
number = {2},
pages = {676--681},
doi = {10.1021/nl403938g}
}
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MLA
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Kvashnin, Alexander G., et al. “Phase Diagram of Quasi-Two-Dimensional Carbon, From Graphene to Diamond.” Nano Letters, vol. 14, no. 2, Jan. 2014, pp. 676-681. https://doi.org/10.1021/nl403938g.