Nano Letters, volume 15, issue 6, pages 3692-3696

Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut

Loredana Protesescu ^{1, 2}

Sergii Yakunin ^{1, 2}

Maryna I. Bodnarchuk ^{1, 2}

Franziska Krieg ^{1, 2}

R. Caputo ¹

Christopher H. Hendon ³

Ruo Yu Yang ³

Aron Walsh ³

Maksym V. Kovalenko ^{1, 2}

Hide authors affiliations Show authors affiliations: 3 affiliations

Institute of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, Vladimir Prelog Weg 1, CH-8093 Zürich, Switzerland |

Laboratory for Thin Films and Photovoltaics, Empa − Swiss Federal Laboratories for Materials Science and Technology, Überlandstrasse 129, CH-8600 Dübendorf, Switzerland |

Centre for Sustainable Chemical Technologies and Department of Chemistry, University of Bath, Bath BA2 7AY, United Kingdom |

Publication type: Journal Article

Publication date: 2015-02-02

American Chemical Society (ACS)

Journal: Nano Letters

Quartile SCImago

Quartile WOS

Impact factor: 10.8

ISSN: 15306984, 15306992

DOI: 10.1021/nl5048779

Copy DOI

PubMed ID: 25633588

General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Bioengineering

Abstract

Metal halides perovskites, such as hybrid organic-inorganic CH3NH3PbI3, are newcomer optoelectronic materials that have attracted enormous attention as solution-deposited absorbing layers in solar cells with power conversion efficiencies reaching 20%. Herein we demonstrate a new avenue for halide perovskites by designing highly luminescent perovskite-based colloidal quantum dot materials. We have synthesized monodisperse colloidal nanocubes (4-15 nm edge lengths) of fully inorganic cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I or mixed halide systems Cl/Br and Br/I) using inexpensive commercial precursors. Through compositional modulations and quantum size-effects, the bandgap energies and emission spectra are readily tunable over the entire visible spectral region of 410-700 nm. The photoluminescence of CsPbX3 nanocrystals is characterized by narrow emission line-widths of 12-42 nm, wide color gamut covering up to 140% of the NTSC color standard, high quantum yields of up to 90%, and radiative lifetimes in the range of 1-29 ns. The compelling combination of enhanced optical properties and chemical robustness makes CsPbX3 nanocrystals appealing for optoelectronic applications, particularly for blue and green spectral regions (410-530 nm), where typical metal chalcogenide-based quantum dots suffer from photodegradation.

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Citations by journals

	50 100 150 200 250 300 350
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 309, 4.39% Journal of Physical Chemistry Letters 309 publications, 4.39%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 290, 4.12% Journal of Physical Chemistry C 290 publications, 4.12%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 254, 3.61% Journal of Materials Chemistry C 254 publications, 3.61%
Advanced Optical Materials	Advanced Optical Materials, 226, 3.21% Advanced Optical Materials 226 publications, 3.21%
Nanoscale	Nanoscale, 217, 3.09% Nanoscale 217 publications, 3.09%
ACS applied materials & interfaces	ACS applied materials & interfaces, 215, 3.06% ACS applied materials & interfaces 215 publications, 3.06%
Chemistry of Materials	Chemistry of Materials, 196, 2.79% Chemistry of Materials 196 publications, 2.79%
ACS Energy Letters	ACS Energy Letters, 165, 2.35% ACS Energy Letters 165 publications, 2.35%
Nano Letters	Nano Letters, 164, 2.33% Nano Letters 164 publications, 2.33%
Advanced Functional Materials	Advanced Functional Materials, 159, 2.26% Advanced Functional Materials 159 publications, 2.26%
ACS Nano	ACS Nano, 158, 2.25% ACS Nano 158 publications, 2.25%
Advanced Materials	Advanced Materials, 154, 2.19% Advanced Materials 154 publications, 2.19%
Journal of the American Chemical Society	Journal of the American Chemical Society, 131, 1.86% Journal of the American Chemical Society 131 publications, 1.86%
ACS Applied Nano Materials	ACS Applied Nano Materials, 126, 1.79% ACS Applied Nano Materials 126 publications, 1.79%
Chemical Engineering Journal	Chemical Engineering Journal, 120, 1.71% Chemical Engineering Journal 120 publications, 1.71%
Small	Small, 105, 1.49% Small 105 publications, 1.49%
Journal of Luminescence	Journal of Luminescence, 91, 1.29% Journal of Luminescence 91 publications, 1.29%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 91, 1.29% Angewandte Chemie - International Edition 91 publications, 1.29%
Angewandte Chemie	Angewandte Chemie, 91, 1.29% Angewandte Chemie 91 publications, 1.29%
Nanomaterials	Nanomaterials, 87, 1.24% Nanomaterials 87 publications, 1.24%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 81, 1.15% Journal of Alloys and Compounds 81 publications, 1.15%
Nature Communications	Nature Communications, 73, 1.04% Nature Communications 73 publications, 1.04%
Chemical Communications	Chemical Communications, 72, 1.02% Chemical Communications 72 publications, 1.02%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 67, 0.95% Journal of Materials Chemistry A 67 publications, 0.95%
Applied Physics Letters	Applied Physics Letters, 60, 0.85% Applied Physics Letters 60 publications, 0.85%
RSC Advances	RSC Advances, 59, 0.84% RSC Advances 59 publications, 0.84%
Nano Research	Nano Research, 58, 0.82% Nano Research 58 publications, 0.82%
Nanotechnology	Nanotechnology, 58, 0.82% Nanotechnology 58 publications, 0.82%
Nano Energy	Nano Energy, 57, 0.81% Nano Energy 57 publications, 0.81%
	50 100 150 200 250 300 350

Citations by publishers

	500 1000 1500 2000 2500
American Chemical Society (ACS)	American Chemical Society (ACS), 2134, 30.35% American Chemical Society (ACS) 2134 publications, 30.35%
Wiley	Wiley, 1351, 19.21% Wiley 1351 publications, 19.21%
Elsevier	Elsevier, 1080, 15.36% Elsevier 1080 publications, 15.36%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 966, 13.74% Royal Society of Chemistry (RSC) 966 publications, 13.74%
Springer Nature	Springer Nature, 437, 6.22% Springer Nature 437 publications, 6.22%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 222, 3.16% Multidisciplinary Digital Publishing Institute (MDPI) 222 publications, 3.16%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 172, 2.45% American Institute of Physics (AIP) 172 publications, 2.45%
IOP Publishing	IOP Publishing, 155, 2.2% IOP Publishing 155 publications, 2.2%
Optical Society of America	Optical Society of America, 92, 1.31% Optical Society of America 92 publications, 1.31%
American Physical Society (APS)	American Physical Society (APS), 45, 0.64% American Physical Society (APS) 45 publications, 0.64%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 26, 0.37% American Association for the Advancement of Science (AAAS) 26 publications, 0.37%
Frontiers Media S.A.	Frontiers Media S.A., 25, 0.36% Frontiers Media S.A. 25 publications, 0.36%
Walter de Gruyter	Walter de Gruyter, 24, 0.34% Walter de Gruyter 24 publications, 0.34%
IEEE	IEEE, 22, 0.31% IEEE 22 publications, 0.31%
Taylor & Francis	Taylor & Francis, 17, 0.24% Taylor & Francis 17 publications, 0.24%
Pleiades Publishing	Pleiades Publishing, 14, 0.2% Pleiades Publishing 14 publications, 0.2%
The Electrochemical Society	The Electrochemical Society, 14, 0.2% The Electrochemical Society 14 publications, 0.2%
Chinese Physical Society	Chinese Physical Society, 14, 0.2% Chinese Physical Society 14 publications, 0.2%
Japan Society of Applied Physics	Japan Society of Applied Physics, 13, 0.18% Japan Society of Applied Physics 13 publications, 0.18%
Materials Research Society	Materials Research Society, 10, 0.14% Materials Research Society 10 publications, 0.14%
World Scientific	World Scientific, 9, 0.13% World Scientific 9 publications, 0.13%
SPIE	SPIE, 7, 0.1% SPIE 7 publications, 0.1%
Cambridge University Press	Cambridge University Press, 7, 0.1% Cambridge University Press 7 publications, 0.1%
Opto-Electronic Advances	Opto-Electronic Advances, 7, 0.1% Opto-Electronic Advances 7 publications, 0.1%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 7, 0.1% Proceedings of the National Academy of Sciences (PNAS) 7 publications, 0.1%
The Chemical Society of Japan	The Chemical Society of Japan, 5, 0.07% The Chemical Society of Japan 5 publications, 0.07%
Korean Ceramic Society	Korean Ceramic Society, 4, 0.06% Korean Ceramic Society 4 publications, 0.06%
Oxford University Press	Oxford University Press, 3, 0.04% Oxford University Press 3 publications, 0.04%
Beilstein-Institut	Beilstein-Institut, 2, 0.03% Beilstein-Institut 2 publications, 0.03%
	500 1000 1500 2000 2500

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Protesescu L. et al. Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut // Nano Letters. 2015. Vol. 15. No. 6. pp. 3692-3696.

GOST all authors (up to 50) Copy

Protesescu L., Yakunin S., Bodnarchuk M. I., Krieg F., Caputo R., Hendon C. H., Yang R. Yu., Walsh A., Kovalenko M. V. Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut // Nano Letters. 2015. Vol. 15. No. 6. pp. 3692-3696.

RIS |

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TY - JOUR

DO - 10.1021/nl5048779

UR - https://doi.org/10.1021/nl5048779

TI - Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut

T2 - Nano Letters

AU - Protesescu, Loredana

AU - Yakunin, Sergii

AU - Bodnarchuk, Maryna I.

AU - Krieg, Franziska

AU - Caputo, R.

AU - Hendon, Christopher H.

AU - Yang, Ruo Yu

AU - Walsh, Aron

AU - Kovalenko, Maksym V.

PY - 2015

DA - 2015/02/02 00:00:00

PB - American Chemical Society (ACS)

SP - 3692-3696

IS - 6

VL - 15

PMID - 25633588

SN - 1530-6984

SN - 1530-6992

ER -

BibTex |

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BibTex Copy

@article{2015_Protesescu,

author = {Loredana Protesescu and Sergii Yakunin and Maryna I. Bodnarchuk and Franziska Krieg and R. Caputo and Christopher H. Hendon and Ruo Yu Yang and Aron Walsh and Maksym V. Kovalenko},

title = {Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut},

journal = {Nano Letters},

year = {2015},

volume = {15},

publisher = {American Chemical Society (ACS)},

month = {feb},

url = {https://doi.org/10.1021/nl5048779},

number = {6},

pages = {3692--3696},

doi = {10.1021/nl5048779}

}

MLA

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MLA Copy

Protesescu, Loredana, et al. “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut.” Nano Letters, vol. 15, no. 6, Feb. 2015, pp. 3692-3696. https://doi.org/10.1021/nl5048779.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Nano Letters

Quartile SCImago

Quartile WOS

Impact factor

10.8

ISSN

15306984 (Print)
15306992 (Electronic)