volume 30 issue 17 pages 4494-4496

Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers

Publication typeJournal Article
Publication date2011-08-03
scimago Q2
wos Q1
SJR0.676
CiteScore5.1
Impact factor2.9
ISSN02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Palladium hydroxide dimers were prepared by reactions of CsOH with monomeric [Pd(NHC)(η3-allyl)Cl] starting materials. The dimers represent species proposed as intermediates in important cross-coupling reactions. These complexes were tested for their catalytic activity in Suzuki–Miyaura coupling and Buchwald–Hartwig aryl amination. The hydroxide complexes were susceptible to hydrogenolysis on exposure to H2 gas. Following H2O elimination and β-hydride elimination of an additional cinnamyl ligand, a Pd(0) species is formed which can react with other available ligands.
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GOST |
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GOST Copy
Egbert J. et al. Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers // Organometallics. 2011. Vol. 30. No. 17. pp. 4494-4496.
GOST all authors (up to 50) Copy
Egbert J., Chartoire A., Slawin A. M. Z., Nolan S. P. Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers // Organometallics. 2011. Vol. 30. No. 17. pp. 4494-4496.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/om200579h
UR - https://doi.org/10.1021/om200579h
TI - Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers
T2 - Organometallics
AU - Egbert, Jonathan
AU - Chartoire, Anthony
AU - Slawin, Alexandra M. Z.
AU - Nolan, Steven P.
PY - 2011
DA - 2011/08/03
PB - American Chemical Society (ACS)
SP - 4494-4496
IS - 17
VL - 30
SN - 0276-7333
SN - 1520-6041
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2011_Egbert,
author = {Jonathan Egbert and Anthony Chartoire and Alexandra M. Z. Slawin and Steven P. Nolan},
title = {Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers},
journal = {Organometallics},
year = {2011},
volume = {30},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/om200579h},
number = {17},
pages = {4494--4496},
doi = {10.1021/om200579h}
}
MLA
Cite this
MLA Copy
Egbert, Jonathan, et al. “Synthesis, Characterization, and Reactivity of N-Heterocyclic Carbene Palladium(II) Hydroxide Dimers.” Organometallics, vol. 30, no. 17, Aug. 2011, pp. 4494-4496. https://doi.org/10.1021/om200579h.