Open Access

Nature Communications, volume 11, issue 1, publication number 2531

Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water

Yiou Wang ^{1, 2}

Xu Liu ²

Xiaoyu Han ^{3, 4}

Robert Godin ^{5, 6}

Jialu Chen ⁷

Wuzong Zhou ⁷

Chaoran Jiang ²

Jamie F Thompson ⁶

Mustafa K Bayazit ^{2, 8}

Stephen A Shevlin ³

Sophia Haussener ⁶

Zhengxiao Guo ^{3, 9, 10, 11}

Junwang Tang ²

Hide authors affiliations Show authors affiliations: 11 affiliations

Chair for Photonics and Optoelectronics, Nano-Institute Munich, Ludwig-Maximilians-Universität München, Munich, Germany |

Department of Chemical Engineering, University College London, London, UK |

Department of Chemistry, University College London, London, UK |

⁴

Department of Chemistry, The University of Manchester, Manchester, UK |

⁵

Department of Chemistry, The University of British Columbia, Kelowna, Canada |

⁶

Department of chemistry, Imperial College London, London, UK |

⁷

School of Chemistry, University of St. Andrews, St. Andrews, UK |

⁸

Nanotechnology Research and Application Center, Sabancı University, Tuzla/İstanbul, Turkey |

⁹

Department of Chemistry, HKU-CAS Joint Laboratory on New Materials, The University of Hong Kong, Hong Kong, China |

¹⁰

Department of Mechanical Engineering, The University of Hong Kong, Hong Kong, china |

¹¹

HKU Zhejiang Institute of Research and Innovation, The University of Hong Kong, Hangzhou, China |

Publication type: Journal Article

Publication date: 2020-05-21

Springer Nature

Journal: Nature Communications

Quartile SCImago

Quartile WOS

Impact factor: 16.6

ISSN: 20411723, 20411723

DOI: 10.1038/s41467-020-16227-3

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General Chemistry

General Biochemistry, Genetics and Molecular Biology

General Physics and Astronomy

Abstract

Solar-driven CO2 reduction by abundant water to alcohols can supply sustainable liquid fuels and alleviate global warming. However, the sluggish water oxidation reaction has been hardly reported to be efficient and selective in CO2 conversion due to fast charge recombination. Here, using transient absorption spectroscopy, we demonstrate that microwave-synthesised carbon-dots (mCD) possess unique hole-accepting nature, prolonging the electron lifetime (t50%) of carbon nitride (CN) by six folds, favouring a six-electron product. mCD-decorated CN stably produces stoichiometric oxygen and methanol from water and CO2 with nearly 100% selectivity to methanol and internal quantum efficiency of 2.1% in the visible region, further confirmed by isotopic labelling. Such mCD rapidly extracts holes from CN and prevents the surface adsorption of methanol, favourably oxidising water over methanol and enhancing the selective CO2 reduction to alcohols. This work provides a unique strategy for efficient and highly selective CO2 reduction by water to high-value chemicals. Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol.

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Citations by journals

	2 4 6 8 10
Chemical Engineering Journal	Chemical Engineering Journal, 10, 4.95% Chemical Engineering Journal 10 publications, 4.95%
Small	Small, 7, 3.47% Small 7 publications, 3.47%
ACS Catalysis	ACS Catalysis, 7, 3.47% ACS Catalysis 7 publications, 3.47%
Nature Communications	Nature Communications, 6, 2.97% Nature Communications 6 publications, 2.97%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 6, 2.97% Applied Catalysis B: Environmental 6 publications, 2.97%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 5, 2.48% Angewandte Chemie - International Edition 5 publications, 2.48%
Angewandte Chemie	Angewandte Chemie, 5, 2.48% Angewandte Chemie 5 publications, 2.48%
ACS Applied Nano Materials	ACS Applied Nano Materials, 4, 1.98% ACS Applied Nano Materials 4 publications, 1.98%
Advanced Materials	Advanced Materials, 4, 1.98% Advanced Materials 4 publications, 1.98%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 4, 1.98% Journal of Physical Chemistry C 4 publications, 1.98%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 1.98% Journal of Materials Chemistry A 4 publications, 1.98%
Catalysts	Catalysts, 3, 1.49% Catalysts 3 publications, 1.49%
Journal of CO2 Utilization	Journal of CO2 Utilization, 3, 1.49% Journal of CO2 Utilization 3 publications, 1.49%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 3, 1.49% Journal of Colloid and Interface Science 3 publications, 1.49%
Nano Energy	Nano Energy, 3, 1.49% Nano Energy 3 publications, 1.49%
Advanced Functional Materials	Advanced Functional Materials, 3, 1.49% Advanced Functional Materials 3 publications, 1.49%
Energy & Fuels	Energy & Fuels, 3, 1.49% Energy & Fuels 3 publications, 1.49%
Chemical Communications	Chemical Communications, 3, 1.49% Chemical Communications 3 publications, 1.49%
ACS Nano	ACS Nano, 3, 1.49% ACS Nano 3 publications, 1.49%
Advanced Science	Advanced Science, 2, 0.99% Advanced Science 2 publications, 0.99%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 0.99% Journal of the American Chemical Society 2 publications, 0.99%
Molecules	Molecules, 2, 0.99% Molecules 2 publications, 0.99%
RSC Advances	RSC Advances, 2, 0.99% RSC Advances 2 publications, 0.99%
ACS Energy Letters	ACS Energy Letters, 2, 0.99% ACS Energy Letters 2 publications, 0.99%
Applied Surface Science	Applied Surface Science, 2, 0.99% Applied Surface Science 2 publications, 0.99%
Colloids and Surfaces A: Physicochemical and Engineering Aspects	Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2, 0.99% Colloids and Surfaces A: Physicochemical and Engineering Aspects 2 publications, 0.99%
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 2, 0.99% International Journal of Hydrogen Energy 2 publications, 0.99%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 2, 0.99% Journal of Materials Science and Technology 2 publications, 0.99%
Journal of Environmental Chemical Engineering	Journal of Environmental Chemical Engineering, 2, 0.99% Journal of Environmental Chemical Engineering 2 publications, 0.99%
	2 4 6 8 10

Citations by publishers

	10 20 30 40 50 60 70
Elsevier	Elsevier, 70, 34.65% Elsevier 70 publications, 34.65%
Wiley	Wiley, 41, 20.3% Wiley 41 publications, 20.3%
American Chemical Society (ACS)	American Chemical Society (ACS), 37, 18.32% American Chemical Society (ACS) 37 publications, 18.32%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 25, 12.38% Royal Society of Chemistry (RSC) 25 publications, 12.38%
Springer Nature	Springer Nature, 14, 6.93% Springer Nature 14 publications, 6.93%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 5, 2.48% Multidisciplinary Digital Publishing Institute (MDPI) 5 publications, 2.48%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.5% Nonferrous Metals Society of China 1 publication, 0.5%
IOP Publishing	IOP Publishing, 1, 0.5% IOP Publishing 1 publication, 0.5%
Oxford University Press	Oxford University Press, 1, 0.5% Oxford University Press 1 publication, 0.5%
Trans Tech Publications	Trans Tech Publications, 1, 0.5% Trans Tech Publications 1 publication, 0.5%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.5% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.5%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.5% OAE Publishing Inc. 1 publication, 0.5%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.5% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.5%
	10 20 30 40 50 60 70

We do not take into account publications without a DOI.
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Wang Y. et al. Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water // Nature Communications. 2020. Vol. 11. No. 1. 2531

GOST all authors (up to 50) Copy

Wang Y., Liu X., Han X., Godin R., Chen J., Zhou W., Jiang C., Thompson J. F., Bayazit M. K., Shevlin S. A., Haussener S., Guo Z., Tang J. Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water // Nature Communications. 2020. Vol. 11. No. 1. 2531

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1038/s41467-020-16227-3

UR - https://doi.org/10.1038/s41467-020-16227-3

TI - Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water

T2 - Nature Communications

AU - Wang, Yiou

AU - Liu, Xu

AU - Han, Xiaoyu

AU - Godin, Robert

AU - Chen, Jialu

AU - Zhou, Wuzong

AU - Jiang, Chaoran

AU - Thompson, Jamie F

AU - Bayazit, Mustafa K

AU - Shevlin, Stephen A

AU - Haussener, Sophia

AU - Guo, Zhengxiao

AU - Tang, Junwang

PY - 2020

DA - 2020/05/21 00:00:00

PB - Springer Nature

IS - 1

VL - 11

SN - 2041-1723

ER -

BibTex

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BibTex Copy

@article{2020_Wang,

author = {Yiou Wang and Xu Liu and Xiaoyu Han and Robert Godin and Jialu Chen and Wuzong Zhou and Chaoran Jiang and Jamie F Thompson and Mustafa K Bayazit and Stephen A Shevlin and Sophia Haussener and Zhengxiao Guo and Junwang Tang},

title = {Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water},

journal = {Nature Communications},

year = {2020},

volume = {11},

publisher = {Springer Nature},

month = {may},

url = {https://doi.org/10.1038/s41467-020-16227-3},

number = {1},

doi = {10.1038/s41467-020-16227-3}

}

Found error?

Publisher

Springer Nature

Journal

Nature Communications

Quartile SCImago

Quartile WOS

Impact factor

16.6

ISSN

20411723 (Print)
20411723 (Electronic)