Open Access
Open access
Nature Communications, volume 13, issue 1, publication number 2049

Topological phase singularities in atomically thin high-refractive-index materials

Kravets Vasyl 2
Tselikov G 1
Stebunov Yury 3
Yakubovsky Dmitry 1
Novikov Sergey 1
Vyshnevyy Andrey 1
Mazitov A. B. 1, 4
Kruglov Ivan 1, 4
Romanov Roman 5
Markeev Andrey M. 1
Arsenin Aleksey 1, 6
Novoselov K. S. 3, 7, 8
Grigorenko Alexander N 2
Publication typeJournal Article
Publication date2022-04-19
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor16.6
ISSN20411723
General Chemistry
General Biochemistry, Genetics and Molecular Biology
General Physics and Astronomy
Abstract

Atomically thin transition metal dichalcogenides (TMDCs) present a promising platform for numerous photonic applications due to excitonic spectral features, possibility to tune their constants by external gating, doping, or light, and mechanical stability. Utilization of such materials for sensing or optical modulation purposes would require a clever optical design, as by itself the 2D materials can offer only a small optical phase delay – consequence of the atomic thickness. To address this issue, we combine films of 2D semiconductors which exhibit excitonic lines with the Fabry-Perot resonators of the standard commercial SiO2/Si substrate, in order to realize topological phase singularities in reflection. Around these singularities, reflection spectra demonstrate rapid phase changes while the structure behaves as a perfect absorber. Furthermore, we demonstrate that such topological phase singularities are ubiquitous for the entire class of atomically thin TMDCs and other high-refractive-index materials, making it a powerful tool for phase engineering in flat optics. As a practical demonstration, we employ PdSe2 topological phase singularities for a refractive index sensor and demonstrate its superior phase sensitivity compared to typical surface plasmon resonance sensors.

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GOST Copy
Ermolaev G. A. et al. Topological phase singularities in atomically thin high-refractive-index materials // Nature Communications. 2022. Vol. 13. No. 1. 2049
GOST all authors (up to 50) Copy
Ermolaev G. A., Voronin K. V., Baranov D. G., Kravets V., Tselikov G., Stebunov Y., Yakubovsky D., Novikov S., Vyshnevyy A., Mazitov A. B., Kruglov I., Zhukov S., Romanov R., Markeev A. M., Arsenin A., Novoselov K. S., Grigorenko A. N., Volkov V. S. Topological phase singularities in atomically thin high-refractive-index materials // Nature Communications. 2022. Vol. 13. No. 1. 2049
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RIS Copy
TY - JOUR
DO - 10.1038/s41467-022-29716-4
UR - https://doi.org/10.1038%2Fs41467-022-29716-4
TI - Topological phase singularities in atomically thin high-refractive-index materials
T2 - Nature Communications
AU - Ermolaev, Georgy A.
AU - Voronin, Kirill V.
AU - Baranov, Denis G.
AU - Tselikov, G
AU - Yakubovsky, Dmitry
AU - Novikov, Sergey
AU - Vyshnevyy, Andrey
AU - Mazitov, A. B.
AU - Zhukov, Sergey
AU - Romanov, Roman
AU - Markeev, Andrey M.
AU - Arsenin, Aleksey
AU - Novoselov, K. S.
AU - Volkov, Valentyn S.
AU - Kravets, Vasyl
AU - Stebunov, Yury
AU - Kruglov, Ivan
AU - Grigorenko, Alexander N
PY - 2022
DA - 2022/04/19 00:00:00
PB - Springer Nature
IS - 1
VL - 13
PMID - 35440544
SN - 2041-1723
ER -
BibTex
Cite this
BibTex Copy
@article{2022_Ermolaev,
author = {Georgy A. Ermolaev and Kirill V. Voronin and Denis G. Baranov and G Tselikov and Dmitry Yakubovsky and Sergey Novikov and Andrey Vyshnevyy and A. B. Mazitov and Sergey Zhukov and Roman Romanov and Andrey M. Markeev and Aleksey Arsenin and K. S. Novoselov and Valentyn S. Volkov and Vasyl Kravets and Yury Stebunov and Ivan Kruglov and Alexander N Grigorenko},
title = {Topological phase singularities in atomically thin high-refractive-index materials},
journal = {Nature Communications},
year = {2022},
volume = {13},
publisher = {Springer Nature},
month = {apr},
url = {https://doi.org/10.1038%2Fs41467-022-29716-4},
number = {1},
doi = {10.1038/s41467-022-29716-4}
}
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