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npj Quantum Materials, volume 7, issue 1, publication number 7

Native point defects and their implications for the Dirac point gap at MnBi2Te4(0001)

Aguilar P Casado 1, 4
Aliev Z S 6, 7
Amiraslanov I R 7, 8
Abdullayev N A 7, 8
Zverev V. N. 9
Babanly M. B. 8, 10
Mamedov N. T. 7
SHIKIN A. M. 5
Arnau A. 2, 11, 12
Vazquez de Parga Amadeo L. 1, 4, 13, 14
Chulkov E.V. 5, 11, 12, 15
Miranda R. M. 1, 4, 13, 14
1
 
Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA-nanociencia), Madrid, Spain
4
 
Departamento de Física de la Materia Condensada, Universidad Autónoma de Madrid, Madrid, Spain
11
 
Departamento de Polímeros y Materiales Avanzados: Física, Química y Tecnología, Facultad de Ciencias Químicas, Universidad del País Vasco UPV/EHU, Donostia-San Sebastián, Spain
13
 
Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Madrid, Spain
14
 
Instituto Nicolás Cabrera, Universidad Autónoma de Madrid, Madrid, Spain
Publication typeJournal Article
Publication date2022-01-14
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor5.7
ISSN23974648
Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Abstract

We study the surface crystalline and electronic structures of the antiferromagnetic topological insulator MnBi2Te4 using scanning tunneling microscopy/spectroscopy (STM/S), micro(μ)-laser angle-resolved photoemission spectroscopy (ARPES), and density functional theory calculations. Our STM images reveal native point defects at the surface that we identify as BiTe antisites and MnBi substitutions. Bulk X-ray diffraction further evidences the presence of the Mn-Bi intermixing. Overall, our characterizations suggest that the defects concentration is nonuniform within crystals and differs from sample to sample. Consistently, the ARPES and STS experiments reveal that the Dirac point gap of the topological surface state is different for different samples and sample cleavages, respectively. Our calculations show that the antiparallel alignment of the MnBi moments with respect to those of the Mn layer can indeed cause a strong reduction of the Dirac point gap size. The present study provides important insights into a highly debated issue of the MnBi2Te4 Dirac point gap.

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Garnica M. et al. Native point defects and their implications for the Dirac point gap at MnBi2Te4(0001) // npj Quantum Materials. 2022. Vol. 7. No. 1. 7
GOST all authors (up to 50) Copy
Garnica M., Otrokov M. M., Aguilar P. C., Klimovskikh I. I., Estyunin D. A., Aliev Z. S., Amiraslanov I. R., Abdullayev N. A., Zverev V. N., Babanly M. B., Mamedov N. T., SHIKIN A. M., Arnau A., Vazquez de Parga A. L., Chulkov E., Miranda R. M. Native point defects and their implications for the Dirac point gap at MnBi2Te4(0001) // npj Quantum Materials. 2022. Vol. 7. No. 1. 7
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Cite this
RIS Copy
TY - JOUR
DO - 10.1038/s41535-021-00414-6
UR - https://doi.org/10.1038%2Fs41535-021-00414-6
TI - Native point defects and their implications for the Dirac point gap at MnBi2Te4(0001)
T2 - npj Quantum Materials
AU - Garnica, Manuela
AU - Otrokov, Mikhail M.
AU - Aguilar, P Casado
AU - Klimovskikh, Ilya I.
AU - Estyunin, Dmitry A.
AU - Amiraslanov, I R
AU - Abdullayev, N A
AU - Zverev, V. N.
AU - Mamedov, N. T.
AU - Arnau, A.
AU - Vazquez de Parga, Amadeo L.
AU - Chulkov, E.V.
AU - Miranda, R. M.
AU - SHIKIN, A. M.
AU - Aliev, Z S
AU - Babanly, M. B.
PY - 2022
DA - 2022/01/14 00:00:00
PB - Springer Nature
IS - 1
VL - 7
SN - 2397-4648
ER -
BibTex
Cite this
BibTex Copy
@article{2022_Garnica,
author = {Manuela Garnica and Mikhail M. Otrokov and P Casado Aguilar and Ilya I. Klimovskikh and Dmitry A. Estyunin and I R Amiraslanov and N A Abdullayev and V. N. Zverev and N. T. Mamedov and A. Arnau and Amadeo L. Vazquez de Parga and E.V. Chulkov and R. M. Miranda and A. M. SHIKIN and Z S Aliev and M. B. Babanly},
title = {Native point defects and their implications for the Dirac point gap at MnBi2Te4(0001)},
journal = {npj Quantum Materials},
year = {2022},
volume = {7},
publisher = {Springer Nature},
month = {jan},
url = {https://doi.org/10.1038%2Fs41535-021-00414-6},
number = {1},
doi = {10.1038/s41535-021-00414-6}
}
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