Open Access
Nanoscale, volume 10, issue 30, pages 14499-14509
Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties
Antonova I. V.
1, 2, 3
,
Erohin Sergey V
4, 5
,
Kvashnin Dmitry
5, 6
,
Olejniczak Andrzej
7, 8
,
Volodin V. A.
1, 2
,
Skuratov V A
8, 9, 10
,
Krasheninnikov Arkady V.
5, 11, 12
,
Sorokin Pavel B.
4, 5, 6
,
Chernozatonskii L A
6
7
Faculty of Chemistry, Nicolaus Copernicus University, Gagarin st. 7, 87-100 Toruń, Poland
|
Publication type: Journal Article
Publication date: 2018-07-03
General Materials Science
Abstract
The morphology and electronic properties of single and few-layer graphene films nanostructured by the impact of heavy high-energy ions have been studied. It is found that ion irradiation leads to the formation of nano-sized pores, or antidots, with sizes ranging from 20 to 60 nm, in the upper one or two layers. The sizes of the pores proved to be roughly independent of the energy of the ions, whereas the areal density of the pores increased with the ion dose. With increasing ion energy (>70 MeV), a profound reduction in the concentration of structural defects (by a factor of 2-5), relatively high mobility values of charge carriers (700-1200 cm2 V-1 s-1) and a transport band gap of about 50 meV were observed in the nanostructured films. The experimental data were rationalized through atomistic simulations of ion impact onto few-layer graphene structures with a thickness matching the experimental samples. We showed that even a single Xe atom with energy in the experimental range produces a considerable amount of damage in the graphene lattice, whereas high dose ion irradiation allows one to propose a high probability of consecutive impacts of several ions onto an area already amorphized by the previous ions, which increases the average radius of the pore to match the experimental results. We also found that the formation of "welded" sheets due to interlayer covalent bonds at the edges and, hence, defect-free antidot arrays is likely at high ion energies (above 70 MeV).
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1 publication, 2.78%
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1 publication, 2.78%
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1 publication, 2.78%
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1
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3
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Citations by publishers
2
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3 publications, 8.33%
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2 publications, 5.56%
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American Institute of Physics (AIP)
1 publication, 2.78%
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Springer Nature
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Springer Nature
1 publication, 2.78%
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2
4
6
8
10
12
14
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- We do not take into account publications that without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Nebogatikova N. A. et al. Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties // Nanoscale. 2018. Vol. 10. No. 30. pp. 14499-14509.
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Nebogatikova N. A., Antonova I. V., Erohin S. V., Kvashnin D., Olejniczak A., Volodin V. A., Skuratov V. A., Krasheninnikov A. V., Sorokin P. B., Chernozatonskii L. A. Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties // Nanoscale. 2018. Vol. 10. No. 30. pp. 14499-14509.
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TY - JOUR
DO - 10.1039/C8NR03062F
UR - https://doi.org/10.1039%2FC8NR03062F
TI - Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties
T2 - Nanoscale
AU - Nebogatikova, Nadezhda A.
AU - Antonova, I. V.
AU - Kvashnin, Dmitry
AU - Olejniczak, Andrzej
AU - Volodin, V. A.
AU - Skuratov, V A
AU - Krasheninnikov, Arkady V.
AU - Sorokin, Pavel B.
AU - Chernozatonskii, L A
AU - Erohin, Sergey V
PY - 2018
DA - 2018/07/03 00:00:00
PB - Royal Society of Chemistry (RSC)
SP - 14499-14509
IS - 30
VL - 10
SN - 2040-3364
SN - 2040-3372
ER -
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@article{2018_Nebogatikova
author = {Nadezhda A. Nebogatikova and I. V. Antonova and Dmitry Kvashnin and Andrzej Olejniczak and V. A. Volodin and V A Skuratov and Arkady V. Krasheninnikov and Pavel B. Sorokin and L A Chernozatonskii and Sergey V Erohin},
title = {Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties},
journal = {Nanoscale},
year = {2018},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {jul},
url = {https://doi.org/10.1039%2FC8NR03062F},
number = {30},
pages = {14499--14509},
doi = {10.1039/C8NR03062F}
}
Cite this
MLA
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Nebogatikova, Nadezhda A., et al. “Nanostructuring few-layer graphene films with swift heavy ions for electronic application: tuning of electronic and transport properties.” Nanoscale, vol. 10, no. 30, Jul. 2018, pp. 14499-14509. https://doi.org/10.1039%2FC8NR03062F.