Open Access
Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii ) catalysts
Jan Philipp Berndt
1
,
Jan-Philipp Berndt
1, 2, 3, 4, 5
,
Yevhenii Radchenko
1, 2, 3, 4, 5
,
Jonathan D. Becker
6
,
Jonathan Becker
4, 5, 7
,
Christian Logemann
4, 5, 6, 7
,
Dhaka R Bhandari
4, 5, 6, 7
,
Radim Hrdina
1, 2, 3, 4, 5
,
Peter R. Schreiner
1, 2, 3, 4, 5
3
Institute of Organic Chemistry
4
35392 Giessen
5
GERMANY
|
6
Institute of Inorganic and Analytical Chemistry, Heinrich-Buff-Ring 17, 35392 Giessen, Germany
|
7
Institute of Inorganic and Analytical Chemistry
Publication type: Journal Article
Publication date: 2019-02-06
scimago Q1
wos Q1
SJR: 2.138
CiteScore: 12.6
Impact factor: 7.4
ISSN: 20416520, 20416539
PubMed ID:
30996919
General Chemistry
Abstract
We report a new strategy for the preparation of dirhodium(ii) complexes with the general formula Rh2(A)4 that allows the isolation of a dirhodium tetracarboxylate complex with a free amino group available for postfunctionalization. The postfunctionalization of this complex enables the incorporation of a variety of functional groups, including double and triple bonds as well as nucleophilic moieties, thus paving the way to new classes of polymeric as well as bifunctional catalysts, and polymetallic complexes. Furthermore, we demonstrate that a urea containing dirhodium(ii) complex enables site-selective nitrenoid insertions by remote hydrogen bonding control.
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Metrics
31
Total citations:
31
Citations from 2025:
5
(16.13%)
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GOST
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Berndt J. P. et al. Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii) catalysts // Chemical Science. 2019. Vol. 10. No. 11. pp. 3324-3329.
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Berndt J. P., Berndt J., Radchenko Y., Becker J. D., Becker J., Logemann C., Bhandari D. R., Hrdina R., Schreiner P. R. Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii) catalysts // Chemical Science. 2019. Vol. 10. No. 11. pp. 3324-3329.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1039/C8SC05733H
UR - https://xlink.rsc.org/?DOI=C8SC05733H
TI - Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii) catalysts
T2 - Chemical Science
AU - Berndt, Jan Philipp
AU - Berndt, Jan-Philipp
AU - Radchenko, Yevhenii
AU - Becker, Jonathan D.
AU - Becker, Jonathan
AU - Logemann, Christian
AU - Bhandari, Dhaka R
AU - Hrdina, Radim
AU - Schreiner, Peter R.
PY - 2019
DA - 2019/02/06
PB - Royal Society of Chemistry (RSC)
SP - 3324-3329
IS - 11
VL - 10
PMID - 30996919
SN - 2041-6520
SN - 2041-6539
ER -
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BibTex (up to 50 authors)
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@article{2019_Berndt,
author = {Jan Philipp Berndt and Jan-Philipp Berndt and Yevhenii Radchenko and Jonathan D. Becker and Jonathan Becker and Christian Logemann and Dhaka R Bhandari and Radim Hrdina and Peter R. Schreiner},
title = {Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii) catalysts},
journal = {Chemical Science},
year = {2019},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {feb},
url = {https://xlink.rsc.org/?DOI=C8SC05733H},
number = {11},
pages = {3324--3329},
doi = {10.1039/C8SC05733H}
}
Cite this
MLA
Copy
Berndt, Jan Philipp, et al. “Site-selective nitrenoid insertions utilizing postfunctionalized bifunctional rhodium(ii) catalysts.” Chemical Science, vol. 10, no. 11, Feb. 2019, pp. 3324-3329. https://xlink.rsc.org/?DOI=C8SC05733H.
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