Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells
German Soto Perez
1, 2
,
Shyantan Dasgupta
3, 4
,
Wiktor Żuraw
3, 5
,
Rosinda Fuentes Pineda
6
,
Konrad Wojciechowski
3, 6
,
Lethy Krishnan Jagadamma
7, 8
,
Ifor D. Samuel
7, 8
,
Neil J. Robertson
1, 2
3
Saule Research Institute, Wroclaw PL 54-130, Poland
|
6
Saule Technologies, Wroclaw PL 54-427, Poland
|
Publication type: Journal Article
Publication date: 2022-04-22
scimago Q1
wos Q1
SJR: 2.462
CiteScore: 16.7
Impact factor: 9.5
ISSN: 20507488, 20507496, 09599428, 13645501
General Chemistry
General Materials Science
Renewable Energy, Sustainability and the Environment
Abstract
Perylene diimide derivatives with different functional groups (OR) in the bay position were synthesised (PDI-1, OR = OC6H4OMe; PDI-2, OR = OC6H4CH2CH2NHBoc; PDI-3, OR = OC6H4CO2Me) and their optoelectronical properties were characterised. The derivatives were applied as alternative electron transport materials (ETMs) to replace the commonly used PCBM in inverted perovskite solar cells (PSCs). Devices with the structure ITO/PTAA/Cs0.04(MA0.17FA0.83)0.96Pb(I0.83Br0.17)3/ETM/Ag (ETM = PCBM or PDI-1, -2 or -3) were fabricated through solution processing techniques. A competitive power conversion efficiency (PCE) of 16.8% was obtained for the PDI-3-based device, which was comparable to the PCBM-based device with PCE of 17.3%. It was found that the electronic nature of the functional groups plays an important role in the charge extraction and band alignment of these small molecular semiconductors.
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Total citations:
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Citations from 2025:
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(19.05%)
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Perez G. S. et al. Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells // Journal of Materials Chemistry A. 2022. Vol. 10. No. 20. pp. 11046-11053.
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Perez G. S., Dasgupta S., Żuraw W., Pineda R. F., Wojciechowski K., Jagadamma L. K., Samuel I. D., Robertson N. J. Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells // Journal of Materials Chemistry A. 2022. Vol. 10. No. 20. pp. 11046-11053.
Cite this
RIS
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TY - JOUR
DO - 10.1039/d2ta01321e
UR - https://xlink.rsc.org/?DOI=D2TA01321E
TI - Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells
T2 - Journal of Materials Chemistry A
AU - Perez, German Soto
AU - Dasgupta, Shyantan
AU - Żuraw, Wiktor
AU - Pineda, Rosinda Fuentes
AU - Wojciechowski, Konrad
AU - Jagadamma, Lethy Krishnan
AU - Samuel, Ifor D.
AU - Robertson, Neil J.
PY - 2022
DA - 2022/04/22
PB - Royal Society of Chemistry (RSC)
SP - 11046-11053
IS - 20
VL - 10
SN - 2050-7488
SN - 2050-7496
SN - 0959-9428
SN - 1364-5501
ER -
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@article{2022_Perez,
author = {German Soto Perez and Shyantan Dasgupta and Wiktor Żuraw and Rosinda Fuentes Pineda and Konrad Wojciechowski and Lethy Krishnan Jagadamma and Ifor D. Samuel and Neil J. Robertson},
title = {Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells},
journal = {Journal of Materials Chemistry A},
year = {2022},
volume = {10},
publisher = {Royal Society of Chemistry (RSC)},
month = {apr},
url = {https://xlink.rsc.org/?DOI=D2TA01321E},
number = {20},
pages = {11046--11053},
doi = {10.1039/d2ta01321e}
}
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Perez, German Soto, et al. “Solution-processable perylene diimide-based electron transport materials as non-fullerene alternatives for inverted perovskite solar cells.” Journal of Materials Chemistry A, vol. 10, no. 20, Apr. 2022, pp. 11046-11053. https://xlink.rsc.org/?DOI=D2TA01321E.
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