Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation
Тип публикации: Journal Article
Дата публикации: 2003-11-21
scimago Q1
wos Q2
БС2
SJR: 0.819
CiteScore: 5.3
Impact factor: 3.1
ISSN: 00219606, 10897690
Physical and Theoretical Chemistry
General Physics and Astronomy
Краткое описание
Strong segregation theory of microphase separation in dilute solutions of associating polyelectrolytes is developed. The driving force of the separation is shown to be a competition between a short-range attraction of associating groups and long-range repulsion of charged groups. We predict that with the increase of polymer concentration single chains first aggregate into spherical clusters of optimum size which can be disordered in space or arranged with the symmetry of the bcc lattice. Further increase of polymer concentration can result in the formation of hexagonal and lamellar structures which precede the physical gelation. The hexagonal and lamellar structures are stable at very small fractions of charged groups on the chains.
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Limberger R. E., Potemkin I. I., Khokhlov A. R. Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation // Journal of Chemical Physics. 2003. Vol. 119. No. 22. pp. 12023-12028.
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Limberger R. E., Potemkin I. I., Khokhlov A. R. Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation // Journal of Chemical Physics. 2003. Vol. 119. No. 22. pp. 12023-12028.
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TY - JOUR
DO - 10.1063/1.1624823
UR - https://doi.org/10.1063/1.1624823
TI - Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation
T2 - Journal of Chemical Physics
AU - Limberger, Roman E.
AU - Potemkin, Igor I
AU - Khokhlov, Alexei R.
PY - 2003
DA - 2003/11/21
PB - AIP Publishing
SP - 12023-12028
IS - 22
VL - 119
SN - 0021-9606
SN - 1089-7690
ER -
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@article{2003_Limberger,
author = {Roman E. Limberger and Igor I Potemkin and Alexei R. Khokhlov},
title = {Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation},
journal = {Journal of Chemical Physics},
year = {2003},
volume = {119},
publisher = {AIP Publishing},
month = {nov},
url = {https://doi.org/10.1063/1.1624823},
number = {22},
pages = {12023--12028},
doi = {10.1063/1.1624823}
}
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Limberger, Roman E., et al. “Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation.” Journal of Chemical Physics, vol. 119, no. 22, Nov. 2003, pp. 12023-12028. https://doi.org/10.1063/1.1624823.
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