Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation
Publication type: Journal Article
Publication date: 2003-11-21
scimago Q1
wos Q2
SJR: 0.819
CiteScore: 5.3
Impact factor: 3.1
ISSN: 00219606, 10897690
Physical and Theoretical Chemistry
General Physics and Astronomy
Abstract
Strong segregation theory of microphase separation in dilute solutions of associating polyelectrolytes is developed. The driving force of the separation is shown to be a competition between a short-range attraction of associating groups and long-range repulsion of charged groups. We predict that with the increase of polymer concentration single chains first aggregate into spherical clusters of optimum size which can be disordered in space or arranged with the symmetry of the bcc lattice. Further increase of polymer concentration can result in the formation of hexagonal and lamellar structures which precede the physical gelation. The hexagonal and lamellar structures are stable at very small fractions of charged groups on the chains.
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26
Total citations:
26
Citations from 2024:
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GOST
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Limberger R. E., Potemkin I. I., Khokhlov A. R. Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation // Journal of Chemical Physics. 2003. Vol. 119. No. 22. pp. 12023-12028.
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Limberger R. E., Potemkin I. I., Khokhlov A. R. Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation // Journal of Chemical Physics. 2003. Vol. 119. No. 22. pp. 12023-12028.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1063/1.1624823
UR - https://doi.org/10.1063/1.1624823
TI - Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation
T2 - Journal of Chemical Physics
AU - Limberger, Roman E.
AU - Potemkin, Igor I
AU - Khokhlov, Alexei R.
PY - 2003
DA - 2003/11/21
PB - AIP Publishing
SP - 12023-12028
IS - 22
VL - 119
SN - 0021-9606
SN - 1089-7690
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2003_Limberger,
author = {Roman E. Limberger and Igor I Potemkin and Alexei R. Khokhlov},
title = {Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation},
journal = {Journal of Chemical Physics},
year = {2003},
volume = {119},
publisher = {AIP Publishing},
month = {nov},
url = {https://doi.org/10.1063/1.1624823},
number = {22},
pages = {12023--12028},
doi = {10.1063/1.1624823}
}
Cite this
MLA
Copy
Limberger, Roman E., et al. “Microphase separation in solutions of associating polyelectrolytes: Strong segregation approximation.” Journal of Chemical Physics, vol. 119, no. 22, Nov. 2003, pp. 12023-12028. https://doi.org/10.1063/1.1624823.
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