Open Access

Physical Review Letters

, том 126 , издание 17 , номер публикации 175501

High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph

Maxim Bykov ^{1, 2}

Timofey Fedotenko ³

Stella Chariton ⁴

Dominique Laniel ³

K. Glazyrin ⁵

M. Hanfland ⁶

Jesse S. Smith ⁷

Jesse J. Smith ⁷

V. Prakapenka ⁴

Mohammad F. Mahmood ²

Alexander F. Goncharov ¹

Alexander Goncharov ¹

A.V. Ponomareva ⁸

Ferenc Tasnádi ⁹

F. Tasnádi ⁹

Alexei I Abrikosov ¹⁰

A.A. Abrikosov ¹⁰

Talha Bin Masood ¹⁰

Ingrid Hotz ¹⁰

Alexander N Rudenko ^{11, 12, 13}

Alexander N. Rudenko ^{11, 12, 13}

Mikhail I Katsnelson ^{11, 13}

M. I. KATSNELSON ^{11, 13}

N.A. Dubrovinskaia ^{3, 9}

Leonid Dubrovinsky ¹⁴

L. Dubrovinsky ¹⁴

Igor A Abrikosov ⁹

I. A. Abrikosov ⁹

Скрыть аффилиации авторов Показать аффилиации авторов: 14 аффилиаций

The Earth and Planets Laboratory, Carnegie Institution for Science, Washington, D.C. 20015, USA |

College of Arts and Science, Howard University, Washington, D.C. 20059, USA |

Material Physics and Technology at Extreme Conditions, Laboratory of Crystallography, University of Bayreuth, 95440 Bayreuth, Germany |

⁴

Center for Advanced Radiation Sources, University of Chicago, Chicago, Illinois 60637, USA |

⁵

Photon Sciences, Deutsches Electronen Synchrotron (DESY), D-22607 Hamburg, Germany |

⁶

European Synchrotron Radiation Facility, 38043 Grenoble Cedex 9, France |

⁷

HPCAT, X-Ray Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA |

⁸

Materials Modeling and Development Laboratory, National University of Science and Technology “MISiS,” 119049 Moscow, Russia |

⁹

Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-58183 Linköping, Sweden |

¹⁰

Department of Science and Technology (ITN), Linköping University, SE-60174 Norrköping, Sweden |

¹¹

Radboud University, Institute for Molecules and Materials, 6525AJ Nijmegen, The Netherlands |

¹²

Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education and School of Physics and Technology, Wuhan University, Wuhan 430072, China |

¹³

Department of Theoretical Physics and Applied Mathematics, Ural Federal University, 620002 Ekaterinburg, Russia |

¹⁴

Bayerisches Geoinstitut, University of Bayreuth, 95440 Bayreuth, Germany |

Тип публикации: Journal Article

Дата публикации: 2021-04-26

American Physical Society (APS)

Physical Review Letters

scimago Q1

wos Q1

БС1

SJR: 2.856

CiteScore: 15.6

Impact factor: 9.0

ISSN: 00319007, 10797114

DOI: 10.1103/PhysRevLett.126.175501

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PubMed ID: 33988447

General Physics and Astronomy

Краткое описание

High pressure chemistry is known to inspire the creation of unexpected new classes of compounds with exceptional properties. Here we report the synthesis at ~90 GPa of novel beryllium polynitrides, monoclinic and triclinic BeN4. The triclinic phase, upon decompression to ambient conditions, transforms into a compound with atomic-thick BeN4 layers interconnected via weak van der Waals bonds consisting of polyacetylene-like nitrogen chains with conjugated {\pi}-systems and Be atoms in square-planar coordination. Theoretical calculations for a single BeN4 layer show that its electronic lattice is described by a slightly distorted honeycomb structure reminiscent of the graphene lattice and the presence of Dirac points in the electronic band structure at the Fermi level. The BeN4 layer, i.e. beryllonitrene, represents a qualitatively new class of 2D materials that can be built of a metal atom and polymeric nitrogen chains and host anisotropic Dirac fermions.

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Оганов Артем

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Bykov M. et al. High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph // Physical Review Letters. 2021. Vol. 126. No. 17. 175501

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Bykov M., Fedotenko T., Chariton S., Laniel D., Glazyrin K., Hanfland M., Smith J. S., Smith J. J., Prakapenka V., Mahmood M. F., Goncharov A. F., Goncharov A., Ponomareva A., Tasnádi F., Tasnádi F., Abrikosov A. I., Abrikosov A., Bin Masood T., Masood T. B., Hotz I., Rudenko A. N., Rudenko A. N., Katsnelson M. I., KATSNELSON M. I., Dubrovinskaia N., Dubrovinsky L., Dubrovinsky L., Abrikosov I. A., Abrikosov I. A. High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph // Physical Review Letters. 2021. Vol. 126. No. 17. 175501

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TY - JOUR

DO - 10.1103/PhysRevLett.126.175501

UR - https://doi.org/10.1103/PhysRevLett.126.175501

TI - High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph

T2 - Physical Review Letters

AU - Bykov, Maxim

AU - Fedotenko, Timofey

AU - Chariton, Stella

AU - Laniel, Dominique

AU - Glazyrin, K.

AU - Hanfland, M.

AU - Smith, Jesse S.

AU - Smith, Jesse J.

AU - Prakapenka, V.

AU - Mahmood, Mohammad F.

AU - Goncharov, Alexander F.

AU - Goncharov, Alexander

AU - Ponomareva, A.V.

AU - Tasnádi, Ferenc

AU - Tasnádi, F.

AU - Abrikosov, Alexei I

AU - Abrikosov, A.A.

AU - Bin Masood, Talha

AU - Masood, Talha Bin

AU - Hotz, Ingrid

AU - Rudenko, Alexander N

AU - Rudenko, Alexander N.

AU - Katsnelson, Mikhail I

AU - KATSNELSON, M. I.

AU - Dubrovinskaia, N.A.

AU - Dubrovinsky, Leonid

AU - Dubrovinsky, L.

AU - Abrikosov, Igor A

AU - Abrikosov, I. A.

PY - 2021

DA - 2021/04/26

PB - American Physical Society (APS)

IS - 17

VL - 126

PMID - 33988447

SN - 0031-9007

SN - 1079-7114

ER -

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@article{2021_Bykov,

author = {Maxim Bykov and Timofey Fedotenko and Stella Chariton and Dominique Laniel and K. Glazyrin and M. Hanfland and Jesse S. Smith and Jesse J. Smith and V. Prakapenka and Mohammad F. Mahmood and Alexander F. Goncharov and Alexander Goncharov and A.V. Ponomareva and Ferenc Tasnádi and F. Tasnádi and Alexei I Abrikosov and A.A. Abrikosov and Talha Bin Masood and Talha Bin Masood and Ingrid Hotz and Alexander N Rudenko and Alexander N. Rudenko and Mikhail I Katsnelson and M. I. KATSNELSON and N.A. Dubrovinskaia and Leonid Dubrovinsky and L. Dubrovinsky and Igor A Abrikosov and I. A. Abrikosov},

title = {High-Pressure Synthesis of Dirac Materials: Layered van der Waals Bonded BeN4 Polymorph},

journal = {Physical Review Letters},

year = {2021},

volume = {126},

publisher = {American Physical Society (APS)},

month = {apr},

url = {https://doi.org/10.1103/PhysRevLett.126.175501},

number = {17},

pages = {175501},

doi = {10.1103/PhysRevLett.126.175501}

}

Издатель

American Physical Society (APS)

Журнал

Physical Review Letters

scimago Q1

wos Q1

БС1

SJR

2.856

CiteScore

15.6

Impact factor

9.0

ISSN

00319007 (Print)

10797114 (Electronic)

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