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volume 27 issue 19 pages 6537

Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates

Publication typeJournal Article
Publication date2022-10-03
scimago Q1
wos Q2
SJR0.865
CiteScore8.6
Impact factor4.6
ISSN14203049
Organic Chemistry
Drug Discovery
Physical and Theoretical Chemistry
Pharmaceutical Science
Molecular Medicine
Analytical Chemistry
Chemistry (miscellaneous)
Abstract

New CoII substituted malonate field-induced molecular magnets {[Rb6Co3(cpdc)6(H2O)12]∙6H2O}n (1) and [Cs2Co(cpdc)2(H2O)6]n (2) (where cpdc2− stands for cyclopropane-1,1-dicarboxylic acid dianions) were synthesized. Both compounds contain mononuclear bischelate fragments {CoII(cpdc)2(H2O)2}2− where the quasi-octahedral cobalt environment (CoO6) is complemented by water molecules in apical positions. The alkali metal atoms play the role of connectors between the bischelate fragments to form 3D and 2D polymeric structures for 1 and 2, respectively. Analysis of dc magnetic data using the parametric Griffith Hamiltonian for high-spin CoII supported by ab initio calculations revealed that both compounds have an easy axis of magnetic anisotropy. Compounds 1 and 2 exhibit slow magnetic relaxation under an external magnetic field (HDC = 1000 and 1500 Oe, respectively).

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Matyukhina A. K. et al. Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates // Molecules. 2022. Vol. 27. No. 19. p. 6537.
GOST all authors (up to 50) Copy
Matyukhina A. K., Zorina-Tikhonova E. N., Goloveshkin A. S., Babeshkin K. A., Efimov N. N., Kiskin M. A., Eremenko I. L. Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates // Molecules. 2022. Vol. 27. No. 19. p. 6537.
RIS |
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RIS Copy
TY - JOUR
DO - 10.3390/molecules27196537
UR - https://doi.org/10.3390/molecules27196537
TI - Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates
T2 - Molecules
AU - Matyukhina, Anna K
AU - Zorina-Tikhonova, Ekaterina N.
AU - Goloveshkin, Alexander S.
AU - Babeshkin, Konstantin A
AU - Efimov, Nikolay N.
AU - Kiskin, Mikhail A.
AU - Eremenko, Igor L.
PY - 2022
DA - 2022/10/03
PB - MDPI
SP - 6537
IS - 19
VL - 27
PMID - 36235074
SN - 1420-3049
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2022_Matyukhina,
author = {Anna K Matyukhina and Ekaterina N. Zorina-Tikhonova and Alexander S. Goloveshkin and Konstantin A Babeshkin and Nikolay N. Efimov and Mikhail A. Kiskin and Igor L. Eremenko},
title = {Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates},
journal = {Molecules},
year = {2022},
volume = {27},
publisher = {MDPI},
month = {oct},
url = {https://doi.org/10.3390/molecules27196537},
number = {19},
pages = {6537},
doi = {10.3390/molecules27196537}
}
MLA
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MLA Copy
Matyukhina, Anna K., et al. “Field-Induced Slow Magnetic Relaxation in CoII Cyclopropane-1,1-dicarboxylates.” Molecules, vol. 27, no. 19, Oct. 2022, p. 6537. https://doi.org/10.3390/molecules27196537.