volume 21 issue 46 pages 16344-16348

General Route to Cyclobutadiene Rhodium Complexes

Publication typeJournal Article
Publication date2015-09-21
scimago Q1
wos Q2
SJR0.981
CiteScore6.7
Impact factor3.7
ISSN09476539, 15213765
General Chemistry
Catalysis
Organic Chemistry
Abstract

Cyclobutadiene rhodium complexes bear high potential for applications in organometallic synthesis and catalysis. We have found that the cyclobutadiene complexes with substitutionally labile p‐xylene ligands [(C4R4)Rh(p‐xylene)]+ can be synthesized in one step from the commercially available bis(ethylene) complex [{(C2H4)2RhCl}2], p‐xylene, and internal alkynes. The replacement of p‐xylene by various ligands provides a general access to other [(C4R4)Rh] compounds, such as [(C4R4)RhCl]x, [(C4R4)RhL3]+, [(C4R4)Rh(C5H5)], and [(C4R4)Rh(arene)]+. Complex [(C4Et4)Rh(p‐xylene)]+ also catalyzes an unusual cycloisomerization of a 1,11‐dien‐6‐yne into a bicyclic diene.

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GOST |
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GOST Copy
Perekalin D. S. et al. General Route to Cyclobutadiene Rhodium Complexes // Chemistry - A European Journal. 2015. Vol. 21. No. 46. pp. 16344-16348.
GOST all authors (up to 50) Copy
Perekalin D. S., Shvydkiy N. V., Nelyubina Y. V., Kudinov A. R. General Route to Cyclobutadiene Rhodium Complexes // Chemistry - A European Journal. 2015. Vol. 21. No. 46. pp. 16344-16348.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1002/chem.201503270
UR - https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270
TI - General Route to Cyclobutadiene Rhodium Complexes
T2 - Chemistry - A European Journal
AU - Perekalin, Dmitry S
AU - Shvydkiy, Nikita V
AU - Nelyubina, Yulia V.
AU - Kudinov, Alexander R
PY - 2015
DA - 2015/09/21
PB - Wiley
SP - 16344-16348
IS - 46
VL - 21
PMID - 26387565
SN - 0947-6539
SN - 1521-3765
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2015_Perekalin,
author = {Dmitry S Perekalin and Nikita V Shvydkiy and Yulia V. Nelyubina and Alexander R Kudinov},
title = {General Route to Cyclobutadiene Rhodium Complexes},
journal = {Chemistry - A European Journal},
year = {2015},
volume = {21},
publisher = {Wiley},
month = {sep},
url = {https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270},
number = {46},
pages = {16344--16348},
doi = {10.1002/chem.201503270}
}
MLA
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MLA Copy
Perekalin, Dmitry S., et al. “General Route to Cyclobutadiene Rhodium Complexes.” Chemistry - A European Journal, vol. 21, no. 46, Sep. 2015, pp. 16344-16348. https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/chem.201503270.