Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions
Тип публикации: Journal Article
Дата публикации: 2008-01-01
scimago Q2
wos Q3
БС2
SJR: 0.459
CiteScore: 3.9
Impact factor: 2.0
ISSN: 14341948, 10990682
Inorganic Chemistry
Краткое описание
The synthesis of complexes of the general formula Cl2Ru(SIMes)(L)(3-phenylinden-1-ylidene) (5, L = PCy3; 6, L = py; and 7, L = PPh3) from Cl2Ru(PR3)2(3-phenylinden-1-ylidene) (2a, R = Ph; 2b, R = Cy) is reported. This family of olefin metathesis catalysts was fully characterized (1H, 13C and 31P NMR spectroscopy and elemental analysis) and provided excellent activity in the ring-opening metathesis polymerization of 1,5-cyclooctadiene and the ring-closing metathesis of diethyl diallylmalonate. Comparison with the corresponding benzylidene-containing catalysts, 1a,c and 8b, established the decisive role of the carbene ligand on the procedure of the reaction and led to the observation of an unusual catalytic phenomenon, here called “self-inhibition”.(© Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2008)
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Monsaert S. et al. Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions // European Journal of Inorganic Chemistry. 2008. Vol. 2008. No. 3. pp. 432-440.
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Monsaert S., Drozdzak R., Dragutan V., Dragutan I., Verpoort F. Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions // European Journal of Inorganic Chemistry. 2008. Vol. 2008. No. 3. pp. 432-440.
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TY - JOUR
DO - 10.1002/ejic.200700879
UR - https://doi.org/10.1002/ejic.200700879
TI - Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions
T2 - European Journal of Inorganic Chemistry
AU - Monsaert, Stijn
AU - Drozdzak, Renata
AU - Dragutan, Valerian
AU - Dragutan, Ileana
AU - Verpoort, Francis
PY - 2008
DA - 2008/01/01
PB - Wiley
SP - 432-440
IS - 3
VL - 2008
SN - 1434-1948
SN - 1099-0682
ER -
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@article{2008_Monsaert,
author = {Stijn Monsaert and Renata Drozdzak and Valerian Dragutan and Ileana Dragutan and Francis Verpoort},
title = {Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions},
journal = {European Journal of Inorganic Chemistry},
year = {2008},
volume = {2008},
publisher = {Wiley},
month = {jan},
url = {https://doi.org/10.1002/ejic.200700879},
number = {3},
pages = {432--440},
doi = {10.1002/ejic.200700879}
}
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MLA
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Monsaert, Stijn, et al. “Indenylidene‐Ruthenium Complexes Bearing Saturated N‐Heterocyclic Carbenes: Synthesis and Catalytic Investigation in Olefin Metathesis Reactions.” European Journal of Inorganic Chemistry, vol. 2008, no. 3, Jan. 2008, pp. 432-440. https://doi.org/10.1002/ejic.200700879.