European Physical Journal E

, том 4 , издание 1 , страницы 93-101

Stiffness and conformations of molecular bottle-brushes strongly adsorbed on a flat surface

Тип публикации: Journal Article

Дата публикации: 2001-01-01

Springer Nature

European Physical Journal E

scimago Q3

wos Q3

БС2

SJR: 0.396

CiteScore: 3.7

Impact factor: 2.2

ISSN: 12928941, 1292895X

DOI: 10.1007/s101890170147

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General Chemistry

Biophysics

Biotechnology

General Materials Science

Surfaces and Interfaces

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Abstract:A theory of the conformational behavior and analysis of the persistence length of molecular bottle-brushes strongly adsorbed on a flat surface in a good solvent is presented. For long enough side chains we have shown that the adsorption of a small fraction of side chains already leads to significant increase of the stiffness and drastic conformational changes of the brush in comparison with the 3D case. For a symmetrical distribution of the adsorbed side chains with respect to the backbone, the equilibrium conformation of the brush is close to a rod-like one due to the very large stiffness of the molecule. Under certain conditions the excluded-volume interactions of the side chains of an asymmetrical brush can lead to its bending or twisting in spiral. The obtained results are in good agreement with computer simulations.

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5 цитирований

Хохлов Алексей

д.ф.-м.н., проф., академик, Российская академия наук

822 публикации, 21 447 цитирований

Индекс Хирша: 72

Московский государственный университет имени М.В. Ломоносова

Институт элементоорганических соединений им. А.Н. Несмеянова РАН

Области научных интересов

Наука о полимерах

Теория и компьютерное моделирование мягких сред

3 цитирования

Субботин Андрей

д.ф.-м.н.

76 публикаций, 1 443 цитирования, 5 рецензий

Индекс Хирша: 21

Институт физической химии и электрохимии им. А.Н. Фрумкина РАН

Институт нефтехимического синтеза им. А.В. Топчиева РАН

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Механика и реология полимеров

Физика сплошных сред

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Электроспиннинг

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Potemkin I. I., Khokhlov A. R., Reineker P. Stiffness and conformations of molecular bottle-brushes strongly adsorbed on a flat surface // European Physical Journal E. 2001. Vol. 4. No. 1. pp. 93-101.

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TY - JOUR

DO - 10.1007/s101890170147

UR - https://doi.org/10.1007/s101890170147

TI - Stiffness and conformations of molecular bottle-brushes strongly adsorbed on a flat surface

T2 - European Physical Journal E

AU - Potemkin, I I

AU - Khokhlov, A R

AU - Reineker, P.

PY - 2001

DA - 2001/01/01

PB - Springer Nature

SP - 93-101

IS - 1

VL - 4

SN - 1292-8941

SN - 1292-895X

ER -

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@article{2001_Potemkin,

author = {I I Potemkin and A R Khokhlov and P. Reineker},

title = {Stiffness and conformations of molecular bottle-brushes strongly adsorbed on a flat surface},

journal = {European Physical Journal E},

year = {2001},

volume = {4},

publisher = {Springer Nature},

month = {jan},

url = {https://doi.org/10.1007/s101890170147},

number = {1},

pages = {93--101},

doi = {10.1007/s101890170147}

}

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Potemkin, I. I., et al. “Stiffness and conformations of molecular bottle-brushes strongly adsorbed on a flat surface.” European Physical Journal E, vol. 4, no. 1, Jan. 2001, pp. 93-101. https://doi.org/10.1007/s101890170147.