volume 58 issue 13 pages 8645-8656

Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane.

A F Smolyakov 1, 2, 3
I A Godovikov 1
J R Shakirova 4
I S Podkorytov 5
Publication typeJournal Article
Publication date2019-06-19
scimago Q1
wos Q1
SJR0.958
CiteScore7.4
Impact factor4.7
ISSN00201669, 1520510X
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The first example of trinuclear copper(I) and silver(I) pyrazolates adducts with a tertiary diphosphine (Ph2PCH2PPh2) retaining trimeric [MPz]3 core is reported. Despite rather strong M-P bonding, the complexes are able to undergo the dissociation of one M-P bond leading to the "merry-go-round" movement of P atoms over the M3 triangle. The copper complex displays emission from 1MLCT and 3MLCT states. The triplet and singlet states are separated by a relatively small energy gap (1080 cm-1) that triggers the thermally activated delayed fluorescence (TADF) behavior and leads to the worthy quantum yield of 41% at 298 K. The silver complex in the solid state and frozen solution shows dual emission originating from the 1IL and 3MLCT states that is dictated by the much higher energy difference between the emissive singlet and triplet as well as by the essentially different nature of these states.
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Titov A. A. et al. Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane. // Inorganic Chemistry. 2019. Vol. 58. No. 13. pp. 8645-8656.
GOST all authors (up to 50) Copy
Titov A. A., Filippov O. A., Smolyakov A. F., Godovikov I. A., Godovikov I. A., Shakirova J. R., Shakirova J. R., Tunik S. P., Podkorytov I. S., Shubina E. S. Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane. // Inorganic Chemistry. 2019. Vol. 58. No. 13. pp. 8645-8656.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.inorgchem.9b00991
UR - https://pubs.acs.org/doi/10.1021/acs.inorgchem.9b00991
TI - Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane.
T2 - Inorganic Chemistry
AU - Titov, Aleksei A
AU - Filippov, Oleg A.
AU - Smolyakov, A F
AU - Godovikov, Ivan A
AU - Godovikov, I A
AU - Shakirova, Julia R
AU - Shakirova, J R
AU - Tunik, Sergey P.
AU - Podkorytov, I S
AU - Shubina, Elena S.
PY - 2019
DA - 2019/06/19
PB - American Chemical Society (ACS)
SP - 8645-8656
IS - 13
VL - 58
PMID - 31247857
SN - 0020-1669
SN - 1520-510X
ER -
BibTex |
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BibTex (up to 50 authors) Copy
@article{2019_Titov,
author = {Aleksei A Titov and Oleg A. Filippov and A F Smolyakov and Ivan A Godovikov and I A Godovikov and Julia R Shakirova and J R Shakirova and Sergey P. Tunik and I S Podkorytov and Elena S. Shubina},
title = {Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane.},
journal = {Inorganic Chemistry},
year = {2019},
volume = {58},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://pubs.acs.org/doi/10.1021/acs.inorgchem.9b00991},
number = {13},
pages = {8645--8656},
doi = {10.1021/acs.inorgchem.9b00991}
}
MLA
Cite this
MLA Copy
Titov, Aleksei A., et al. “Luminescent Complexes of the Trinuclear Silver(I) and Copper(I) Pyrazolates Supported with Bis(diphenylphosphino)methane..” Inorganic Chemistry, vol. 58, no. 13, Jun. 2019, pp. 8645-8656. https://pubs.acs.org/doi/10.1021/acs.inorgchem.9b00991.