том 38 издание 16 страницы 3151-3158

Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination

A. S. Peregudov 1
Gleb L Denisov 3
Denis Chusov 1, 3, 4
Тип публикацииJournal Article
Дата публикации2019-08-07
scimago Q2
wos Q1
БС1
SJR0.676
CiteScore5.1
Impact factor2.9
ISSN02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Краткое описание
The η6-fluorene cyclopentadienyl complexes [(η5-C5R5)M(η6-fluorene)](SbF6)2 (1: M = Co, R = Me; 2a: M = Rh, R = H; 2b: M = Ir, R = H) were synthesized by the iodide abstraction from [(η5-C5R5)MI2]n with AgSbF6 in the presence of fluorene. The procedure is also suitable for the synthesis of the indenyl derivatives [(η5-indenyl)M(η6-fluorene)](SbF6)2 (3a: M = Rh; 3b: M = Ir) starting from [(η5-indenyl)MI2]n. The structures of [1](SbF6)2 and [2b](SbF6)2 were determined by X-ray diffraction. The rhodium complex [2a](SbF6)2 readily undergoes the replacement of the fluorene ligand by mesitylene, being more reactive than the benzene derivative [CpRh(η6-C6H6)](SbF6)2. According to experimental data and DFT calculations, the fluorene elimination proceeds via a cascade of η6 → η5 → η1 haptotropic rearrangements. The complex [2b](SbF6)2 (at 1 mol % loading) effectively catalyzes the reductive amination reaction between aldehydes (or ketones) and primary aromatic (or secondary aliphatic) amines in the presence of car...
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ГОСТ |
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Kharitonov V. B. et al. Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination // Organometallics. 2019. Vol. 38. No. 16. pp. 3151-3158.
ГОСТ со всеми авторами (до 50) Скопировать
Kharitonov V. B., Podyacheva E., Nelyubina Y. V., Muratov D. V., Peregudov A. S., Denisov G. L., Chusov D., Loginov D. A. Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination // Organometallics. 2019. Vol. 38. No. 16. pp. 3151-3158.
RIS |
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TY - JOUR
DO - 10.1021/acs.organomet.9b00378
UR - https://doi.org/10.1021/acs.organomet.9b00378
TI - Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination
T2 - Organometallics
AU - Kharitonov, Vladimir B.
AU - Podyacheva, Evgeniya
AU - Nelyubina, Yulia V.
AU - Muratov, Dmitry V.
AU - Peregudov, A. S.
AU - Denisov, Gleb L
AU - Chusov, Denis
AU - Loginov, Dmitry A.
PY - 2019
DA - 2019/08/07
PB - American Chemical Society (ACS)
SP - 3151-3158
IS - 16
VL - 38
SN - 0276-7333
SN - 1520-6041
ER -
BibTex |
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@article{2019_Kharitonov,
author = {Vladimir B. Kharitonov and Evgeniya Podyacheva and Yulia V. Nelyubina and Dmitry V. Muratov and A. S. Peregudov and Gleb L Denisov and Denis Chusov and Dmitry A. Loginov},
title = {Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination},
journal = {Organometallics},
year = {2019},
volume = {38},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.organomet.9b00378},
number = {16},
pages = {3151--3158},
doi = {10.1021/acs.organomet.9b00378}
}
MLA
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Kharitonov, Vladimir B., et al. “Fluorene Complexes of Group 9 Metals: Fluorene Effect and Application for Reductive Amination.” Organometallics, vol. 38, no. 16, Aug. 2019, pp. 3151-3158. https://doi.org/10.1021/acs.organomet.9b00378.